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| Open AccessSqueezed light from an oscillator measured at the rate of oscillation
The authors demonstrated an unprecedented level of polarization squeezing of light generated by an atomic ensemble, and a new regime of continuous quantum measurements on a macroscopic material oscillator.
- Christian Bærentsen
- , Sergey A. Fedorov
- & Eugene S. Polzik
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Article
| Open AccessDeterministic positioning and alignment of a single-molecule exciton in plasmonic nanodimer for strong coupling
Realising single molecule strong coupling with plasmons achieving both deterministic molecule positioning and dipole alignment with the mode field has proven challenging so far. Here, the authors fill this gap by placing a single molecular emitter in the gap centre of an Au nanodimer system.
- Renming Liu
- , Ming Geng
- & Lin Wu
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Article
| Open AccessOptical vectorial-mode parity Hall effect: a case study with cylindrical vector beams
This study uses a customized metasurface to unveil a distinct parity Hall effect in degenerate optical vectorial modes. This work realizes the advances in meta-devices and showcases new possibilities for manipulating optical fields based on parity.
- Changyu Zhou
- , Weili Liang
- & Xiaocong Yuan
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Article
| Open AccessPlasma electron acceleration driven by a long-wave-infrared laser
The laser pulses that drive most laser wakefield accelerators have wavelengths near 1 micrometer and peak power > 100 terawatts. Here, the authors drive plasma wakes with 10 micrometer, 2-terawatt pulses, yielding relativistic electron beams with a collimated, narrow-energy-bandwidth component.
- R. Zgadzaj
- , J. Welch
- & M. C. Downer
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Article
| Open AccessCoherent electric field control of orbital state of a neutral nitrogen-vacancy center
Color centers in diamond have been proposed as a link between remote superconducting units in hybrid quantum systems, where their orbital degree of freedom is utilized. Here the authors report coherent electric-field control of the orbital state of a neutral NV center in diamond.
- Hodaka Kurokawa
- , Keidai Wakamatsu
- & Hideo Kosaka
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Article
| Open AccessCoherent optical coupling to surface acoustic wave devices
Surface acoustic wave devices enable modern electronics and are desirable for quantum systems. Here the authors access and control these devices optically, enabling high acoustic quality factors, materials spectroscopy, and hybrid quantum systems.
- Arjun Iyer
- , Yadav P. Kandel
- & William H. Renninger
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Article
| Open AccessCavity-enhanced photon indistinguishability at room temperature and telecom wavelengths
Carbon nanotube-based single photon emitters allow for room-temperature operation, but suffer from vanishing indistinguishability due to strong dephasing. Following a theoretical proposal, the authors tackle the problem experimentally by using a cavity to enhance the photon coherence time and the emission spectral density in the regime of incoherent good cavity-coupling.
- Lukas Husel
- , Julian Trapp
- & Alexander Högele
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Article
| Open AccessGiant magneto-photoluminescence at ultralow field in organic microcrystal arrays for on-chip optical magnetometer
The optical detection of magnetic fields is difficult for low field strengths. Here, the authors show how strong magneto-photoluminescence can be achieved in rubrene microcrystals and demonstrate its application in a magnetometer.
- Hong Wang
- , Baipeng Yin
- & Chuang Zhang
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Article
| Open AccessFrequency comb generation via synchronous pumped χ(3) resonator on thin-film lithium niobate
Here the authors use on-chip amplitude and phase modulation to synchronously pump a resonator on thin-film lithium niobate for frequency comb generation. They find that pulsed pumping significantly mitigates stimulated Raman scattering and improves the overall efficiency of the device.
- Rebecca Cheng
- , Mengjie Yu
- & Marko Lončar
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Article
| Open AccessAnti-resonant acoustic waveguides enabled tailorable Brillouin scattering on chip
Achieving acoustic waveguides with low loss, tailorability, and easy fabrication is a considerable challenge. Here, the authors introduce suspended anti-resonant acoustic waveguides with superior confinement and high selectivity of acoustic modes, supporting both forward and backward SBS on chip.
- Peng Lei
- , Mingyu Xu
- & Xiaopeng Xie
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Article
| Open AccessMiniature computational spectrometer with a plasmonic nanoparticles-in-cavity microfilter array
Conventional spectrometers can be bulky and efforts are being made to develop miniaturised versions. Here, the authors present a miniature computational spectrometer based on silver nanoparticles in Fabry-Pérot microcavities for measuring visible spectra.
- Yangxi Zhang
- , Sheng Zhang
- & A. Ping Zhang
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Article
| Open AccessA statistical resolution measure of fluorescence microscopy with finite photons
Abbe’s diffraction limit has been a defining concept for microscopy. With finite photon, photon noise remains one essential factor yet to be considered in the theoretical resolution limit. Here, the authors introduced information-based resolution limit allowing for photon-considered resolution assessment of various microscopy and super-resolution modalities.
- Yilun Li
- & Fang Huang
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Article
| Open AccessArbitrary engineering of spatial caustics with 3D-printed metasurfaces
Caustics, as a unique type of singularity in wave phenomena, occur in diverse physical systems. Here, the authors realize multi-dimensional customization of caustics with 3D-printed metasurfaces. This arbitrary caustic engineering is poised to bring new revolutions to many domains.
- Xiaoyan Zhou
- , Hongtao Wang
- & Cheng-Wei Qiu
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Article
| Open AccessMulti-site integrated optical addressing of trapped ions
A promising strategy for scaling trapped-ion-based quantum technologies is to use fully integrated optical waveguides to deliver light to numerous ions at multiple sites. Here, the authors. optically address three ions using on-chip waveguides to deliver three distinct wavelengths per ion, and perform Rabi flopping on each ion simultaneously.
- Joonhyuk Kwon
- , William J. Setzer
- & Hayden J. McGuinness
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Article
| Open AccessDelayed room temperature phosphorescence enabled by phosphines
Room-temperature phosphorescence usually occurs immediately after the removal of excitation. Here the authors achieve combined instant and delayed phosphorescence through introduction of phosphines into carbazole emitters.
- Guang Lu
- , Jing Tan
- & Hui Xu
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Article
| Open AccessPhotonic time-crystalline behaviour mediated by phonon squeezing in Ta2NiSe5
Photonic time crystal refers to a material whose dielectric properties oscillate in time. Here the authors theoretically show such behaviour in the excitonic insulator candidate Ta2NiSe5 under optical excitation and use it to explain the enhanced THz reflectivity recently observed in pump-probe experiments
- Marios H. Michael
- , Sheikh Rubaiat Ul Haque
- & Eugene Demler
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Article
| Open AccessDirect programming of confined surface phonon polariton resonators with the plasmonic phase-change material In3SbTe2
Tailored light-matter interaction can be achieved with surface phonon polaritons (SPhPs). Here, Conrads et al. employ the plasmonic phase-change material In3SbTe2 on the polar crystal SiC for direct programming of confined SPhP resonators and study their resonance modes via near-field microscopy.
- Lukas Conrads
- , Luis Schüler
- & Thomas Taubner
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Article
| Open AccessNeural étendue expander for ultra-wide-angle high-fidelity holographic display
All holographic displays and imaging techniques are fundamentally limited by the étendue supported by existing spatial light modulators. Here, the authors report on using artificial intelligence (AI) to learn an étendue expanding element that effectively increases étendue by two orders of magnitude.
- Ethan Tseng
- , Grace Kuo
- & Felix Heide
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Article
| Open AccessHigh-throughput quantum photonic devices emitting indistinguishable photons in the telecom C-band
An efficient way of realising a large number of telecom single-photon emitters for quantum communication is still missing. Here, the authors use a wide-field imaging technique for fast localization of single InAs/InP quantum dots, which are then integrated into circular Bragg grating cavities featuring high single-photon purity and indistinguishability.
- Paweł Holewa
- , Daniel A. Vajner
- & Elizaveta Semenova
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Article
| Open AccessUltrastrong exciton-plasmon couplings in WS2 multilayers synthesized with a random multi-singular metasurface at room temperature
Here, the authors fabricate a metasurface with nanometre-sized plasmonic hotspots that interact coherently with WS2 excitons, achieving ultrastrong exciton-plasmon coupling.
- Tingting Wu
- , Chongwu Wang
- & Yu Luo
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Article
| Open AccessUltrafast photoluminescence and multiscale light amplification in nanoplasmonic cavity glass
This article presents a unique nanocomposite plasmonic-excitonic glass with extraordinary amplified optical properties: ultra-narrow photoluminescence (FWHM = 13 nm) and ultrashort photoluminescence lifetime (90 ps) at room temperature
- Piotr Piotrowski
- , Marta Buza
- & Dorota A. Pawlak
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Article
| Open AccessCorrelation-driven nonequilibrium exciton site transition in a WSe2/WS2 moiré supercell
Correlated insulator states of moire excitons in transition metal dichalcogenide heterostructures have attracted significant attention recently. Here the authors use time-resolved pump-probe spectroscopy to demonstrate the effects of non-equilibrium correlations of moire excitons in WSe2/WS2 heterobilayers.
- Jinjae Kim
- , Jiwon Park
- & Hyunyong Choi
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Article
| Open AccessAn optoacoustic field-programmable perceptron for recurrent neural networks
Optical recurrent neural networks present a unique challenge for photonic machine learning. Here, the authors experimentally show the first optoacoustic recurrent operator based on stimulated Brillouin scattering which may unlock a new class of optical neural networks with recurrent functionality.
- Steven Becker
- , Dirk Englund
- & Birgit Stiller
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Article
| Open AccessExtreme terahertz magnon multiplication induced by resonant magnetic pulse pairs
The authors demonstrate high-order terahertz nonlinear magnonics using two-dimensional coherent spectroscopy, revealing the emergence of seventh-order spin-wave mixing and sixth harmonic magnon generation within an antiferromagnetic orthoferrite.
- C. Huang
- , L. Luo
- & J. Wang
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Article
| Open AccessRoom-temperature quantum emission from interface excitons in mixed-dimensional heterostructures
Interlayer excitons in 2D homo- and heterostructures have been intensively investigated due to their emerging optical properties. Here, the authors report the observation of interface excitons in 1D/2D carbon nanotube/WSe2 heterostructures, showing evidence of photon antibunching at room temperature.
- N. Fang
- , Y. R. Chang
- & Y. K. Kato
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Article
| Open AccessGiant Faraday rotation in atomically thin semiconductors
Here, the authors perform Faraday rotation spectroscopy around the excitonic transitions in hBN-encapsulated WSe2 and MoSe2 monolayers, and interlayer excitons in MoS2 bilayers. They measure a large Verdet constant - 1.9 × 107 deg T−¹cm−¹ for monolayers, and attribute it to the giant oscillator strength and high g-factor of the excitons.
- Benjamin Carey
- , Nils Kolja Wessling
- & Ashish Arora
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Article
| Open AccessObservation of spatiotemporal optical vortices enabled by symmetry-breaking slanted nanograting
A microscale platform composed of a slanted nanograting is experimentally demonstrated to efficiently generate spatiotemporal optical vortex. This approach paves the way towards an integrated system for ultrafast pulse shaping.
- Pengcheng Huo
- , Wei Chen
- & Ting Xu
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Article
| Open AccessFast joint parity measurement via collective interactions induced by stimulated emission
Parity detection is essential in quantum error correction. Here, authors propose a reliable joint parity measurement (JPM) scheme inspired by stimulated emission and experimentally implement the weight-2(4) JPM scheme in a tunable coupling superconducting circuit, which shows comparable performance to the standard CNOT-gate based scheme.
- Sainan Huai
- , Kunliang Bu
- & Yicong Zheng
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Article
| Open AccessIntercavity polariton slows down dynamics in strongly coupled cavities
Band engineering in optics allows the design of unconventional forms of light with potential optoelectronic applications. Here, the authors realize slow-light intercavity polaritons in an array of coupled cavities, the photonic architecture enables the spatial segregation of photons and excitons
- Yesenia A. García Jomaso
- , Brenda Vargas
- & Giuseppe Pirruccio
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Article
| Open AccessLarge area single crystal gold of single nanometer thickness for nanophotonics
2D metallic single crystals are sought after for nanophotonic applications, but their synthesis remains challenging. Here, the authors report an atomic level precision etching method to fabricate large-area crystalline gold flakes with nanometre thickness, showing enhanced plasmonic and nonlinear optical properties.
- Chenxinyu Pan
- , Yuanbiao Tong
- & Pan Wang
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Article
| Open AccessDynamic switching from coherent perfect absorption to parametric amplification in a nonlinear spoof plasmonic waveguide
The authors propose a nonlinear spoof plasmonic waveguide to realize coherent perfect absorption and parametric amplification at the same frequency, which opens a new route to actively modulate the electromagnetic waves with giant amplification-to-absorption contrast.
- Wen Yi Cui
- , Jingjing Zhang
- & Tie Jun Cui
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Article
| Open AccessHyperbolic metamaterial empowered controllable photonic Weyl nodal line semimetals
One-dimensional photonic crystals provide a platform to modulate Weyl quasiparticles with properties of bound states in the continuum both dynamically (transition and rotation) and topologically (singularities in bilateral drumhead surface states).
- Shengyu Hu
- , Zhiwei Guo
- & Hong Chen
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Article
| Open AccessEfficient excitation and control of integrated photonic circuits with virtual critical coupling
The authors achieve enhanced cavity loading using complex-frequency excitations that can tailor on-demand the effective coupling rate in a microring resonator by precisely controlling the temporal evolution of the incident pulses.
- Jakob Hinney
- , Seunghwi Kim
- & Michal Lipson
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Article
| Open AccessRaman time-delay in attosecond transient absorption of strong-field created krypton vacancy
The advent of isolated attosecond XUV pulse sources marks a new era in attosecond science, pivotal for the investigation of core electron dynamics. Here the authors discover that the coherent Raman coupling between the cation states leads to extra timedelay between different transition channels by applying the attosecond transient absorption spectroscopy on the investigation of complex dynamics of strong field ionization of Krypton.
- Li Wang
- , Guangru Bai
- & Zengxiu Zhao
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Article
| Open AccessDemonstration of hypergraph-state quantum information processing
Usual multiqubit entangled states can be described using the graph formalism, where each edge connects only two qubits. Here, instead, the authors use a reprogrammable silicon photonics chip to showcase preparation, verification and processing of arbitrary four-qubit hypergraph states, where hyperedges describe entanglement within a subset of many qubits.
- Jieshan Huang
- , Xudong Li
- & Jianwei Wang
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Article
| Open AccessDefect-induced helicity dependent terahertz emission in Dirac semimetal PtTe2 thin films
Defect engineering of topological materials provides an avenue for the controllable manipulation of optoelectronic properties. Here, the authors introduce a defect gradient into a Dirac semimetal to control the Berry curvature dipole-driven THz emission in the material.
- Zhongqiang Chen
- , Hongsong Qiu
- & Xuefeng Wang
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Article
| Open AccessTunable anisotropic van der Waals films of 2M-WS2 for plasmon canalization
Anisotropic light-matter excitations in van der Waals materials are expected to have an impact on nanophotonics applications. Here, the authors report the observation of canalized in-plane mid-infrared plasmons in the semimetallic phase of WS2 and demonstrate their electrical tunability via ion intercalation.
- Qiaoxia Xing
- , Jiasheng Zhang
- & Hugen Yan
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Article
| Open AccessUniversal control of a bosonic mode via drive-activated native cubic interactions
Manipulating quantum information encoded in a bosonic mode requires sizeable and controllable nonlinearities, but superconducting devices’ strong nonlinearities are normally static. Here, the authors use a SNAIL to suppress static nonlinearities and use drive-dependent ones to reach universal control of a bosonic mode.
- Axel M. Eriksson
- , Théo Sépulcre
- & Simone Gasparinetti
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Article
| Open AccessHigh performance artificial visual perception and recognition with a plasmon-enhanced 2D material neural network
Here, the authors demonstrate a low-power neuromorphic visual architecture based on a plasmon-enhanced 2D semiconductor phototransistor array, showing high-speed sensing, preprocessing and image recognition functionalities.
- Tian Zhang
- , Xin Guo
- & Linjun Li
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Article
| Open AccessPoincaré sphere trajectory encoding metasurfaces based on generalized Malus’ law
Polarization serves as an excellent information encoding carrier. Here, authors expand the metasurface encoding dimensionality of polarization information by engineering the Poincaré Sphere trajectory with generalized Malus’ law, unveiling new opportunities for advanced polarization optics.
- Zi-Lan Deng
- , Meng-Xia Hu
- & Andrea Alù
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Article
| Open AccessHermitian and non-Hermitian topology from photon-mediated interactions
Topological properties of a photonic environment are crucial to engineer robust photon-mediated interactions between quantum emitters. Here, the authors find general theorems on the topology of photon-mediated interactions, unveiling the phenomena of topological preservation and reversal.
- Federico Roccati
- , Miguel Bello
- & Angelo Carollo
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Article
| Open AccessCavity-coupled telecom atomic source in silicon
T centers in silicon are promising candidates for quantum applications yet suffer from weak optical transitions. Here, by integrating with a silicon nanocavity, the authors demonstrate an enhancement of the photon emission rate for a single T center.
- Adam Johnston
- , Ulises Felix-Rendon
- & Songtao Chen
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Article
| Open AccessUltra-compact exciton polariton modulator based on van der Waals semiconductors
Miniaturized and efficient optical modulators are desired for data transmission, processing and communication. Here, the authors report the fabrication of exciton-polariton Mach–Zehnder modulators based on thin WS2 waveguides with a footprint of ~30 μm², modulation ratio up to −6.20 dB and nanosecond response times.
- Seong Won Lee
- , Jong Seok Lee
- & Su-Hyun Gong
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Article
| Open AccessTime-of-flight detection of terahertz phonon-polariton
Polaritons, light-matter hybridized quasiparticles, are the fundamental excitation of strong coupling systems and are widely applicable in information technologies. Here the authors applied the concept of time-of-flight measurement in terahertz induced second harmonic generation experiments in various systems to comprehensively study the dispersion relation of phonon-polaritons and reveal potential spin-lattice couplings.
- Tianchuang Luo
- , Batyr Ilyas
- & Nuh Gedik
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Article
| Open AccessRoom-temperature strong coupling in a single-photon emitter-metasurface system
Interfacing single-photon emitters (SPEs) with high-finesse cavities can prevent decoherence processes, especially at elevated temperature, but its implementation remains challenging. Here, the authors report room-temperature strong coupling of SPEs in hexagonal boron nitride with a dielectric cavity based on bound states in the continuum, showing a Rabi splitting of ~ 4 meV.
- T. Thu Ha Do
- , Milad Nonahal
- & Son Tung Ha
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Article
| Open AccessBroadband angular spectrum differentiation using dielectric metasurfaces
Metasurfaces processing incoming images have been proposed in the context of real space operations. Here, the authors demonstrate mathematical operations, such as differentiation, on the angular spectrum of an image using metasurfaces, which can be used to enhance spectral features of an image.
- Ming Deng
- , Michele Cotrufo
- & Lin Chen
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Article
| Open AccessRetinal photoisomerization versus counterion protonation in light and dark-adapted bacteriorhodopsin and its primary photoproduct
Malakar et al. investigate the photochemical dynamics in the isomerization of bacteriorhodopsin light and dark-adapted forms and in the first photocycle intermediate, K. The results prompt a reevaluation of the counter ion model, revealing that a different protonation then that shown in the classic quadrupole so far considered must be employed to account for the experimental data.
- Partha Malakar
- , Samira Gholami
- & Sanford Ruhman
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Comment
| Open AccessBerkSEL: A scale-invariant laser beyond the Schawlow-Townes two-mirror strategy
I argue that a surface emitting laser that remains single mode irrespective of its size, a scale-invariant laser, should of necessity also waste light at the edge. This is a fundamental departure from the Schawlow-Townes two-mirror strategy that keeps light away from mirrors and edges to preserve gain and minimize loss. The strategy was implemented in the recent discovery of the Berkeley Surface Emitting Laser (BerkSEL).
- Boubacar Kanté
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Article
| Open AccessSpectral-temporal-spatial customization via modulating multimodal nonlinear pulse propagation
The authors introduce a method for modulating the multimodal nonlinear pulse propagation in fibers by controlled bending, achieving a tunable broadband high-peak-power femtosecond light source that could empower nonlinear imaging and spectroscopy.
- Tong Qiu
- , Honghao Cao
- & Sixian You
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