Abstract
In recent years, important progress has been made towards encoding and processing quantum information in the large Hilbert space of bosonic modes. Mechanical resonators have several practical advantages for this purpose, because they confine many high-quality-factor modes into a small volume and can be easily integrated with different quantum systems. However, it is challenging to create direct interactions between different mechanical modes that can be used to emulate quantum gates. Here we demonstrate an in situ tunable beamsplitter-type interaction between several mechanical modes of a high-overtone bulk acoustic-wave resonator. The engineered interaction is mediated by a parametrically driven superconducting transmon qubit, and we show that it can be tailored to couple pairs or triplets of phononic modes. Furthermore, we use this interaction to demonstrate the Hong–Ou–Mandel effect between phonons. Our results lay the foundations for using phononic systems as quantum memories and platforms for quantum simulations.
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Main
Mechanical degrees of freedom are a particularly interesting quantum platform, as they involve the collective motion of massive particles, can have long coherence times and can be combined with many other quantum systems1. Circuit quantum acoustodynamics (cQAD) systems, where a superconducting qubit is coupled to gigahertz-frequency acoustic modes, have recently been engineered2,3,4 and used to demonstrate the generation and measurement of non-trivial quantum states4,5,6,7,8 and entanglement between mechanical modes9. Due to the small mode volumes, low crosstalk and high coherence times of acoustic modes, cQAD devices have become the target platform of recent proposals for the realization of a quantum random-access memory10 as well as fault-tolerant quantum computing architectures11,12. In particular, cQAD devices that incorporate high-overtone bulk acoustic-wave resonators (HBARs) can take advantage of the HBAR’s large effective mass and multimode properties, making them excellent platforms for the implementation of bosonic quantum simulations13,14,15, bosonic encodings16,17, quantum metrology applications18 and fundamental studies of quantum mechanical interference phenomena between phonons19,20,21.
An important yet currently missing tool for the realization of these applications is the generation of a phononic iSWAP gate, which is an operation that allows for a direct exchange of quanta between mechanical modes. This can be engineered via a beamsplitter interaction, a coupling mechanism that has already been studied between photonic modes22,23, in optomechanical systems24, in trapped ions25, between mechanical resonators in the classical regime19,26 and between travelling mechanical waves21. When brought to the quantum regime, this phononic beamsplitter interaction will not only become a building block of quantum computing architectures10,11,12 but will also offer new possibilities for the simulation of complex quantum systems and the phononic realization of quantum-optics-type experiments that have so far been mostly explored with photonic systems.
In this work, we demonstrate a beamsplitter interaction between multiple phonon modes of an HBAR coupled to a superconducting transmon qubit. We create this interaction by applying two off-resonant drives on the qubit27 such that it acts as a nonlinear mixing element. We first study the effects of this bichromatic driving through qubit spectroscopy, observe the generation of multiple sidebands and show how these sidebands mediate the desired beamsplitter coupling. Having realized this interaction, we then perform time-domain experiments to demonstrate both iSWAP and \(\sqrt{{\rm{i}}{{{\rm{SWAP}}}}}\) gates, subsequently using the latter to demonstrate entanglement between two acoustic overtone modes of our HBAR. Furthermore, by choosing another parameter regime, we create an interference between three phononic modes and explore the multimode dynamics governing the system. Finally, we utilize the beamsplitter interaction to exchange multiple excitations between the modes and observe the Hong–Ou–Mandel interference21,22,25,28,29,30 between macroscopic mechanical modes.
The device used in this work is a cQAD system where a superconducting qubit is flip-chip bonded to an HBAR7. The qubit is a three-dimensional transmon with a frequency of ωq = 2π × 5.97 GHz, an energy relaxation time of T1 = 9.5 µs, a Ramsey decoherence time of \({T}_{2}^{\,* }\) = 7.2 µs and an anharmonicity α = 2π × 218 MHz. The longitudinal free spectral range (FSR) of the HBAR is approximately 2π × 12.63 MHz, and the two subsystems are coupled through a piezoelectric transducer that mediates a Jaynes–Cummings (JC) interaction with a coupling strength of gm = 2π × 257 kHz. The device is housed in a three-dimensional aluminium cavity, which we use to both shield the qubit from its environment and read its state via the dispersive interaction between the qubit and the cavity. Supplementary Table I provides a full list of system parameters.
Although the cQAD device used in this work has been previously studied in both dispersive5 and resonant coupling regimes6, here we focus on direct multimode interactions that arise when two parametric drives are applied to the qubit. The Hamiltonian of our system in the presence of these drives is given by
where we assume gm to be real. Here the first two terms describe the qubit as an anharmonic mode with lowering operator q. The sum over phonon modes m = a, b, c… with frequencies ωm and lowering operators m includes their energies as well as their JC interaction with the qubit. The last term, given by \({H}_{{{{\rm{qd}}}}}=\left({\varOmega }_{1}{{\rm{e}}}^{-{\rm{i}}{\omega }_{1}t}+{\varOmega }_{2}{{\rm{e}}}^{-{\rm{i}}{\omega }_{2}t}\right){q}^{{\dagger} }+{{{\rm{h.c.}}}}\), describes two off-resonant microwave drives applied to the qubit with frequencies ω1 = ωq + 2π × 492.5 MHz and ω2 ≈ ω1 + FSR. The drives, together with two modes a and b, can participate in a four-wave mixing process mediated by the Josephson nonlinearity of the superconducting qubit10,27,31. In particular, when the resonance condition Δ21 ≡ ω2 − ω1 = ωb − ωa is satisfied, equation (1) leads to a bilinear coupling between the phonon modes. Even though this picture is quantitatively accurate for large phonon–phonon detunings and small drive strengths, we now present a framework that extends this picture to address the case of large drive strengths and small phonon–phonon detunings. Furthermore, our analysis readily lends itself to systems with many bosonic modes by explicitly considering processes involving multiple drive photons.
We first consider only the effect of the drives on the qubit itself. Due to transmon anharmonicity, going into the displaced frame of the drives results in a modulated a.c. Stark shift of the qubit frequency given by (Supplementary Section V)
with the dimensionless drive strengths ξj = Ωj/Δj, where Δj = ωj − ωq for j ∈ {1, 2}. This shift has a time-independent as well as a time-dependent contribution, the latter arising from the beating between the two drives, which modulates the qubit frequency with Δ21. As usual for a frequency-modulated system32,33,34 (Fig. 1a), this gives rise to the appearance of multiple qubit sidebands separated by Δ21, whose amplitudes are given by \({J}_{n}\left(\frac{\Lambda }{{\Delta }_{21}}\right)\). Here Jn(x) is the Bessel function of the first kind for a given sideband number n, and Λ = −4αξ1ξ2. We note that due to the interplay of the parametric drives with the third energy level of the qubit, HStark acquires a correction, which we derive using time-independent perturbation theory (Supplementary Section III). In the following, we use the corrected value for the modulation depth, which we label as Λ′. Furthermore, we will use the shorthand \({J}_{n}={J}_{n}\left(\frac{{\Lambda }^{{\prime} }}{{\Delta }_{21}}\right)\).
We experimentally confirm these effects via two-tone spectroscopy. Specifically, we sweep a weak probe signal across the qubit frequency with the off-resonant drives turned on and subsequently measure the resulting qubit population using dispersive readout. As expected, we find multiple resonances separated by Δ21 with different peak heights, which are the qubit sidebands described above (Fig. 1b). The measured steady-state population of the qubit is quantitatively described in the same way as in a regular qubit spectroscopy experiment35, with the probe strength adjusted by the sideband amplitude (Fig. 1b, continuous black line). After repeating the measurement for a range of parametric drive strengths ξ1ξ2 (ξ1 = ξ2), we find the result shown in Fig. 1c, where we observe multiple diagonal lines spaced in frequency by Δ21 and with varying intensities. These qubit sidebands shift to lower frequencies with increasing drive power, as expected from the Stark shift described by the first term in equation (2).
The JC interaction between the driven qubit and phonon modes results in anti-crossings where the frequency of a sideband matches that of a phonon mode (Fig. 1c,d). However, the effective qubit–phonon coupling strength is scaled by the amplitude of the sideband closest to the phonon mode. Therefore, the gap of the anti-crossing will be reduced from 2gm to 2Jngm, as indicated for n = 0 (Fig. 1d).
In the dispersive regime, where all the qubit sidebands and phonon modes are far detuned, it is useful to enter the interaction picture of the sideband-mediated qubit–phonon coupling via the Schrieffer–Wolff transformation36. After applying the rotating-wave approximation, we can identify two effects in the resulting effective Hamiltonian. First, there is a frequency shift in the phonon modes, due to their hybridization with the qubit37, such that the phonon frequency in the presence of the driven qubit is ωm + δm with
where \({\tilde{\Delta }}_{m}={\omega }_{m}-{\tilde{\omega }}_{q}\) is the detuning between phonon mode m and the Stark-shifted qubit. We see that a phonon mode’s frequency shift is dominated by the sideband for which the denominator in equation (3) is the smallest. Second, although the Schrieffer–Wolff transformation typically eliminates the JC coupling term between the qubit and phonons, in our case, it also gives rise to phonon–phonon coupling terms. For example, the coupling between two neighbouring phonon modes b and c is given by gbc(b†c + bc†), with
when Δ21 = ωc − ωb + δc − δb, such that this term remains after the rotating-wave approximation. Here δb,c refer to the frequency shift of phonons b and c as described by equation (3). Similarly, the next-nearest-neighbouring phonon modes a and c experience a coupling of gac(a†c + ac†), with
when 2Δ21 = ωc − ωa + δc − δa.
The numerator of equation (4), which contains the product of two successive Bessel functions, represents the physical process of the qubit converting one photon between the parametric drives. The frequency conversion of the drive photons compensates for the energy difference between the phonon modes, making the beamsplitter interaction resonant. Interestingly, the effective coupling strength for this process does not become larger monotonically with increasing drive strengths ξ1ξ2. Instead, the speed of the single-photon conversion is reduced in favour of multiphoton processes, for example, converting two drive photons to bridge the energy gap between the phonon modes with a frequency difference of 2Δ21 (equation (5)). Supplementary Sections II and IV provide a more detailed derivation of the different transformations and their effects on the system Hamiltonian.
The dependence of the qubit sidebands on the Bessel functions is what allows us to choose different combinations of coupling strengths between the phonon modes and frequency shifts throughout this work. Naively, it might seem that due to the equal frequency spacing of the phonon modes, one cannot choose interactions between only a subset to be resonant. However, this is not the case. For instance, by choosing an appropriate modulation depth Λ′/Δ21, we can choose the amplitude of J0 to be larger than those of the neighbouring sidebands, namely, J1 and J−1. According to equation (3), the phonon mode closest to the zeroth sideband will shift by a larger amount \((\propto {J}_{0}^{2})\) than the adjacent phonon modes \((\propto {J}_{1}^{2},\,{J}_{-1}^{2})\), giving rise to a unique frequency spacing between the two phonon modes equal to Δ21 and promoting a beamsplitter interaction between them (Fig. 2a). If, on the other hand, we choose a regime where J0 = J1 = − J−1, the three phonon modes a, b and c adjacent in frequency to the n = −1, 0 and 1 sidebands, respectively, will be equally shifted, promoting beamsplitter interactions between these three modes. Note that in the latter case, the next-nearest-neighbour modes a and c are coupled via a two-photon conversion described by equation (5).
We now experimentally investigate the first case of coupling between only the two modes b and c (Fig. 2a). By choosing appropriate drive strengths ξ1,2, we set the modulation depth to Λ′/Δ21 = 0.610 ± 0.001 such that J0 = 0.91 ± 0.01 and J1 = 0.29 ± 0.01. Here the errors are propagated from uncertainties in the independent measurement of system parameters (Supplementary Table I). Our experimental protocol starts with swapping an excitation from the qubit into mode c using the resonant JC interaction. Note that we use a third microwave drive, far detuned from the parametric drives, to independently adjust the frequency of the qubit for this swap operation and to compensate the Stark shift of the qubit from the parametric drives during the beamsplitter interaction to set \({\tilde{\varDelta }}_{{b}}\) = 2π × 1.0 MHz ± 17 kHz. We then turn on the parametric drives for a variable time τBS (Fig. 2b). Afterwards, the qubit has a finite excited-state population due to the off-resonant drives. We reset the qubit to its ground state by swapping its residual population to an ancillary phonon mode detuned by several FSRs from the modes of interest6. Finally, we swap the excitation from mode b or c into the qubit and measure its excited-state population.
Repeating this experiment for different values of Δ21, we observe the expected chevron pattern produced by a beamsplitter-type interaction between the two modes (Fig. 2c). Here we vary Δ21 by only about ±1%, such that we can treat the modulation depth as constant. When Δ21 matches the unique detuning between the two modes Δ, we satisfy the resonance condition for the four-wave mixing process, and the exchange of quanta between the modes becomes most efficient. This occurs for a modulation frequency of (Δ21 − FSR) = −2π × 44 kHz, which matches our prediction from equation (3). We plot the phonon-mode populations for Δ21 = Δ (Fig. 2d) and fit them each to a decaying oscillation, yielding a beamsplitter coupling rate of gbc = 2π × 15.6 ± 0.1 kHz. Note that the contrast for the oscillation in phonon mode b is slightly lower than that for phonon mode c. This is a result of the different decay rates between the two phonon modes, as well as a small but finite leakage to the next phonon mode, namely, m−1 (Fig. 2a). The microscopic origin of the different decay rates for different HBAR modes is a subject of ongoing research38.
At the time τBS = π/4gBS = 8.0 μs (Fig. 2d, dashed line), the interaction becomes a 50:50 beamsplitter or \(\sqrt{{\rm{i}}{{{\rm{SWAP}}}}}\) gate, which creates an entangled state between the two phonon modes. We experimentally confirm this by performing two-qubit state tomography on the resulting state (Fig. 2e). Here, in contrast to the data shown in Fig. 2c,d, we measure the observables of both phonon modes in the same sequence, thereby accessing joint two-mode observables necessary for full-state tomography. To quantify the created entanglement, we compute an overlap of the reconstructed density matrix with the maximally entangled state \(\left\vert bc\right\rangle =(\left\vert 01\right\rangle +{{\rm{e}}}^{{\rm{i}}\phi }\left\vert 10\right\rangle )/\sqrt{2}\) of FBell = 0.69 ± 0.01, with ϕ chosen to optimize FBell. This confirms the presence of entanglement between the two phonon modes. We attribute the difference between the reconstructed density matrix and the maximally entangled state to phonon decay during the \(\sqrt{{\rm{i}}{{{\rm{SWAP}}}}}\) gate and an imperfect state preparation of the initial Fock state in mode c. Supplementary Section VI provides details on the tomography procedure.
Having demonstrated a beamsplitter interaction between the two phonon modes, we now move on to create simultaneous interactions between three modes. To that end, we tune the modulation depth to Λ′/Δ21 = 1.430 ± 0.003 such that J0 = J1 = −J−1 = 0.55 ± 0.01. In this regime, phonon modes a, b and c are equally shifted such that Δcb = Δba ≡ Δ. This is schematically shown in Fig. 3a. In this case, phonon-mode pairs (b, c) and (a, b) are coupled via equation (4), whereas the mode pair (a, c) is coupled via equation (5), with ∣gab∣ ≈ ∣gbc∣ ≈ ∣gac∣.
To explore the dynamics of this three-mode coupling scheme, we extend the experiment presented in Fig. 2. Specifically, we load an excitation into phonon mode b and turn on the parametric drives, thereby activating beamsplitter interactions between all the three modes, and finally measure their population. As before, we sweep the interaction time τBS and the modulation frequency Δ21, with \({\tilde{\varDelta }}_{b}\) = 2π × 1.0 MHz ± 17 kHz. The results are shown in Fig. 3b,c. Although they show the expected qualitative aspects of the excitation swapping between all the three modes, we observe two interesting features. First, when Δ21 = Δ, the initial excitation in mode b flows to modes a and c with approximately equal rates (Fig. 3d). However, the excitation does not fully swap to modes a and c, which is visible from the reduced oscillation contrast (Fig. 3d, grey-shaded area). Although counterintuitive at first, this is the expected behaviour of a three-mode system with coupling between all the mode pairs. The coupling between modes a and c hybridizes them into new normal modes with frequencies shifted by the coupling strength. As a result, the coupling between these normal modes and mode b is no longer resonant, resulting in the reduced oscillation contrast we observe. We note that the frequency of the population exchange observed in Fig. 3d, namely, 2π × 64 ± 1.5 kHz, is in good agreement with theoretical calculations.
The second observation is that the data in Fig. 3c for mode a are approximately the mirror image of mode c with respect to Δ21 − Δ = 0. For instance, when Δ21 − Δ > 0 (Δ21 − Δ < 0), the initial excitation in mode b predominantly flows to mode a (c). Although the roles of modes a and c are symmetric when Δ21 = Δ, this symmetry is broken away from the resonance condition due to the coupling between modes a and c and the resulting normal-mode splitting. Supplementary Section VIII presents a detailed explanation for both these effects.
Although we present experimental details on two interesting values of modulation depth, we note that we can tune from one regime to the other by changing the drive powers, thereby observing a gradual change in both coupling strength and relative detuning (Fig. 3e). To acquire the effective interaction strengths between the three modes as well as their respective phonon frequency shifts, we perform the experiment shown in Fig. 3b,c for different values of ξ1ξ2, thereby varying Λ′/Δ21. We then fit the measured phonon populations to a set of coupled equations of motion with beamsplitter couplings gmk and relative phonon detunings δmk as free parameters (m, k ∈ {a, b, c}). Supplementary Section VII provide details on the fitting procedure. The fit results are plotted alongside equations (3)–(5) with no free parameters (Fig. 3e) and show good agreement between experiment and theory. The observed difference between ∣gab∣ and ∣gbc∣ is a result of the different relative contributions from the sidebands in equation (4) depending on the position of the phonon modes involved. In particular, the observed reduction in ∣gab∣ and ∣gbc∣ for larger modulation depths, as well as the accompanying increase in ∣gac∣, are well captured by theory. We emphasize that previous works have only investigated a much smaller range of modulation depths; therefore, these effects were not evident16,27,31,39.
So far, we have studied the two- and three-mode coupling regimes for the particular case where a single phononic quantum is shared between all of the participating modes. We now investigate the interplay of two quanta during a beamsplitter operation. We first create a |cb〉 = |11〉 state in modes b and c by repeatedly exciting the qubit and swapping its excitation into each mode7. We then turn on the two-mode beamsplitter interaction and subsequently measure the resulting phonon Fock-state distributions of either mode by monitoring the qubit population during a resonant qubit–phonon JC interaction, as shown in previous work7 (Fig. 4a). As an example, the results for a beamsplitter time of τBS = 6.7 μs are shown in Fig. 4b. Here, to optimize the coupling strength and reduce the residual JC interaction with the qubit, we use a slightly larger qubit–phonon detuning of \({\tilde{\Delta }}_{b}\) = 2π × 1.2 MHz ± 17 kHz and modulation depth of Λ′/Δ21 = 0.850 ± 0.002, resulting in gbc = 2π × 18.5 ± 0.8 kHz.
The Hong–Ou–Mandel effect predicts that the outcome of this experiment should depend on whether or not the two phonons are distinguishable. If they are, no interference between them will occur and the excitations will be equally shared between the two phonon modes. On the other hand, if they are indistinguishable, both excitations will bunch in one of the two phonon modes after the beamsplitter. To experimentally confirm this, we compare the probability of the bunched (P20 + P02) with that of the anti-bunched outcome (P11). We extract the bunched outcome probability from the individual Fock distributions by assigning P02 + P20 to \({P}_{2}^{c}+{P}_{2}^{b}\), where \({P}_{2}^{c(b)}\) is the probability of finding two quanta in mode c (b). Doing so relies on the assumption that our system contains a maximum of two excitations at the start of the beamsplitter interaction and that no additional quanta are added during the sequence. This assumption is justified because the residual thermal population of the phonon modes is less than 1.6% (ref. 40). Under the same assumption, we can put an upper bound on the anti-bunched probability, namely, \({\bar{P}}_{11}=\min ({P}_{1}^{b},{P}_{1}^{\,c})\ge {P}_{11}\). Nevertheless, we still take into account the possibility for leakage into higher Fock states by fitting the qubit–phonon Rabi oscillations for the first five energy levels. The population contribution of these higher levels is 0.01 on average and is then included in the error bars (Fig. 4c).
In Fig. 4c, we show both \({\bar{P}}_{11}\) and P20 + P02 for various beamsplitter interaction times τBS, normalized by the entire two-excitation subspace \({P}_{\Sigma }={P}_{20}+{P}_{02}+{\bar{P}}_{11}\). As expected, the two-excitation manifold of the phonon state in the beginning of the interaction is dominated by |11〉. After τBS = 6.7 µs, which corresponds to a 50:50 beamsplitter (Fig. 4c, vertical dashed line), the joint state is more probably bunched with (P20 + P02)/PΣ = 0.622 ± 0.028.
Although we cannot straightforwardly access the joint Fock distributions of the two phonon modes in our experiment, we can do so in a master equation simulation of our system using independently measured system parameters. The results are plotted as continuous lines in Fig. 4c, showing good agreement between data and theory. The fast oscillations that can be seen for lower interaction times in both theory and experiment arise due to an off-resonant JC interaction with the qubit. This result demonstrates how two apriori distinguishable phononic quanta in modes at different frequencies are made indistinguishable by a frequency-converting coupling, which compensates for the energy difference between the two modes, thereby confirming that the lattice vibrations constituting our phonons display behaviour that cannot be classically described.
In conclusion, we have engineered a direct beamsplitter coupling between two and three distinct mechanical modes of an HBAR. We have used the two-mode interaction to create a phononic \(\sqrt{{\rm{i}}{{{\rm{SWAP}}}}}\) gate, allowing us to generate entanglement between the modes and observe the Hong–Ou–Mandel effect between two phonons. In addition to our experimental data, we have also presented a theoretical model that is in good agreement with our findings. Parametrically driven beamsplitters are being actively studied for the purpose of bosonic quantum computing16,21,39,41. Our work explores a new regime of this interaction, where sidebands generated by a large frequency modulation depth and the conversion of more than one drive photon plays an important role. We find our beamsplitter operation to be limited in speed by the qubit–phonon coupling strength and in fidelity by the phonon lifetimes. Larger values for both these parameters have been observed42,43, though combining both remains a challenge. Nevertheless, on the basis of these recent developments, we expect to be able to improve our device quality in the near future.
Our results provide a fundamental building block for performing quantum-optics-type experiments with massive mechanical excitations6. They also address a key challenge towards realizing a mechanical quantum random-access memory by providing one of two required operations10, the other one being a conditional phase operation31. Furthermore, our technique, in principle, allows for all-to-all coupling between a large number of phononic modes, all compactly hosted within a single physical resonator. This makes our device a hardware-efficient platform for future studies of non-reciprocal interactions19,44 and quantum simulations with bosonic modes13,14,45. Finally, our current system and the concepts discussed here can potentially be extended to single- and two-mode squeezing interactions, enabling Gaussian quantum information processing using mechanical resonators46.
Data availability
All data that support the plots within this paper and other findings of this study are available from the corresponding authors on reasonable request. Source data are provided with this paper.
Code availability
The analysis and simulation codes that support the findings of this study are available from the corresponding authors on request.
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Acknowledgements
We thank E. Verhagen, Y. Zhang and M. Bild for useful discussions. The fabrication of the device was performed at the FIRST cleanroom of ETH Zürich and the BRNC cleanroom of IBM Zürich. We acknowledge support from the Swiss National Science Foundation under grant 200021_204073. M.F. was supported by The Branco Weiss Fellowship—Society in Science, administered by the ETH Zürich.
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Open access funding provided by Swiss Federal Institute of Technology Zurich.
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U.v.L. designed and fabricated the device. U.v.L., I.C.R. and Y.Y. performed the experiments and analysed the data. U.v.L. developed the theoretical model and performed the QuTiP simulations of the experiments. M.F. provided the theory support. Y.C. supervised the work. U.v.L., I.C.R. and Y.C. wrote the paper with input from all authors.
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von Lüpke, U., Rodrigues, I.C., Yang, Y. et al. Engineering multimode interactions in circuit quantum acoustodynamics. Nat. Phys. 20, 564–570 (2024). https://doi.org/10.1038/s41567-023-02377-w
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DOI: https://doi.org/10.1038/s41567-023-02377-w
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