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| Open AccessLong-baseline quantum sensor network as dark matter haloscope
Nearly a century after dark matter was proposed, yet its nature remains elusive. Here, authors present their dark photon dark matter search results using two atomic magnetometer arrays 1700 km apart in large magnetic shields and offer the strongest terrestrial constraint in this mass range to date.
- Min Jiang
- , Taizhou Hong
- & Jiangfeng Du
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Article
| Open AccessMapping a 50-spin-qubit network through correlated sensing
The ability to characterize large and complex nuclear-spin networks could enable quantum applications, such as quantum simulations of many-body physics. Here the authors develop a high-resolution quantum-sensing method and use it to image a network of 50 nuclear spins surrounding a single NV center in diamond.
- G. L. van de Stolpe
- , D. P. Kwiatkowski
- & T. H. Taminiau
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Article
| Open AccessCollectively enhanced Ramsey readout by cavity sub- to superradiant transition
One of the ways excited-state atoms relax to ground state is by emitting radiation. Here the authors demonstrate sub- and super-radiant emission threshold from a cavity-mediated atomic ensemble of Sr atoms.
- Eliot A. Bohr
- , Sofus L. Kristensen
- & Jörg H. Müller
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Article
| Open AccessDistributed quantum sensing of multiple phases with fewer photons
Enhanced sensitivity is a key parameter in quantum metrology. Here the authors demonstrate a distributed quantum phase sensing method that uses fewer photons than the number of parameters needed, and an enhanced quantum sensitivity is achieved.
- Dong-Hyun Kim
- , Seongjin Hong
- & Hyang-Tag Lim
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Article
| Open AccessIsotope engineering for spin defects in van der Waals materials
Isotope engineering can enhance spin coherence of solid-state defects, such as NV centers in diamond but progress for defects in hBN has been limited. Gong et al. report the optimization of isotopes in hBN and demonstrate improved coherence and relaxation times for the negatively charged boron vacancy centers.
- Ruotian Gong
- , Xinyi Du
- & Chong Zu
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Article
| Open AccessEnhancing the sensitivity of atom-interferometric inertial sensors using robust control
Bringing atom-interferometric quantum sensors out of the lab requires the mitigation of several sources of noise. Here, the authors experimentally demonstrate a software-based mitigation method based on tailored error-robust Bragg light-pulse beamsplitters and mirrors.
- Jack C. Saywell
- , Max S. Carey
- & Michael J. Biercuk
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Article
| Open AccessQuantum noise and its evasion in feedback oscillators
Feedback oscillators are a fundamental tool in science and engineering. Here, Loughlin and Sudhir provide a generalized Schawlow-Townes-like formula for quantum-limited feedback oscillators, thus giving a general model to study the fundamental output noise of these devices and techniques to reduce their noise further.
- Hudson A. Loughlin
- & Vivishek Sudhir
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Article
| Open AccessIn situ electron paramagnetic resonance spectroscopy using single nanodiamond sensors
Nanodiamonds containing NV centers are promising electron paramagnetic resonance sensors, however applications are hindered by their random orientation. Qin et al. propose a new protocol that makes the technique insensitive to the sensor’s orientation and present a proof-of-principle in situ demonstration.
- Zhuoyang Qin
- , Zhecheng Wang
- & Jiangfeng Du
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Article
| Open AccessMachine learning assisted vector atomic magnetometry
Multiparameter sensors in quantum optics are often complex due to use of external fields. Here the authors demonstrate a simple single-shot all-optical vector atomic magnetometer based on machine learning for the correspondence of the measured signals and the magnetic field.
- Xin Meng
- , Youwei Zhang
- & Yanhong Xiao
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Article
| Open AccessConstraints on axion-like dark matter from a SERF comagnetometer
Axions are hypothetical particles that constitute leading candidates for the identity of dark matter. Here, the authors improve previous exclusion bounds on axion-like particles in the range of 1.4–200 peV, and report direct terrestrial limits on the coupling of protons and neutrons with axion-like dark matter.
- Itay M. Bloch
- , Roy Shaham
- & Or Katz
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Article
| Open AccessRevealing intrinsic domains and fluctuations of moiré magnetism by a wide-field quantum microscope
By carefully inducing twists or lattice stacking offsets between two adjacent van der Waals crystals, a superlattice potential can be introduced. This Moire lattice offers an incredibly rich physics, ranging from superconductivity to exotic magnetism, depending on van der Waals materials in question. Here, Du et al. study the magnetic domains in twisted CrI3, and show that despite this domain structure, spin fluctuations are spatially homogenous.
- Mengqi Huang
- , Zeliang Sun
- & Chunhui Rita Du
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Article
| Open AccessA lab-based test of the gravitational redshift with a miniature clock network
Testing general relativity with optical clocks is important both as a fundamental test and for metrological applications. Here, a vertical linear array of 5 separate ensembles of strontium atoms trapped in a single optical lattice is used to perform a blinded lab-based test of the gravitational redshift at the mm to cm scale.
- Xin Zheng
- , Jonathan Dolde
- & Shimon Kolkowitz
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Article
| Open AccessNonlinear feedforward enabling quantum computation
The ability to perform nonlinear feedforward operations - that is, conditional operations controlled by nonlinear function of the measurement outcomes - is still a missing ingredient for measurement-based quantum computation. Here, the authors fill this gap using nonlinear electro-optical feedforward and non-Gaussian ancillary states.
- Atsushi Sakaguchi
- , Shunya Konno
- & Akira Furusawa
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Article
| Open AccessCavity-enhanced single-shot readout of a quantum dot spin within 3 nanoseconds
Single-shot readout of optically active spin qubits is typically limited by low photon collection rates and measurement back-action. Here the authors overcome these limitations by using an open cavity approach for single-shot readout of a semiconductor quantum dot and demonstrate record readout time of a few ns.
- Nadia O. Antoniadis
- , Mark R. Hogg
- & Richard J. Warburton
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Article
| Open AccessWitnessing light-driven entanglement using time-resolved resonant inelastic X-ray scattering
Quantum Fisher information is a measure of entanglement that has been previously extracted from equilibrium spectra of quantum materials. Here the authors extend this approach to non-equilibrium systems probed by time-resolved resonant inelastic x-ray scattering measurements.
- Jordyn Hales
- , Utkarsh Bajpai
- & Yao Wang
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Article
| Open AccessSub-micron spin-based magnetic field imaging with an organic light emitting diode
Previous demonstrations of electrically and optically detected magnetic resonance in OLED materials have established these systems as promising candidates for magnetic field sensing. Here the authors present an integrated OLED-based device for magnetic field imaging with sub-micron resolution.
- Rugang Geng
- , Adrian Mena
- & Dane R. McCamey
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Article
| Open AccessQuantum enhanced radio detection and ranging with solid spins
Quantum sensors based on NV centers in diamond are well established, however the sensitivity of detection of high-frequency radio signals has been limited. Here the authors use nanoscale field-focusing to enhance sensitivity and demonstrate ranging for GHz radio signals in an interferometer set-up.
- Xiang-Dong Chen
- , En-Hui Wang
- & Fang-Wen Sun
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Article
| Open AccessToward incompatible quantum limits on multiparameter estimation
In quantum multiparameter estimation, achieving the best precision for each parameter is hindered by the Heisenberg principle. Here, the authors demonstrate how to mitigate this problem by using appropriate probe states.
- Binke Xia
- , Jingzheng Huang
- & Guihua Zeng
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Article
| Open AccessBroadband microwave detection using electron spins in a hybrid diamond-magnet sensor chip
Electron spins in diamond allow magnetometry with high sensitivity, but the bandwidth in the microwave regime is limited to a narrow band around their resonance frequency. Here, the authors solve this problem by coupling the spins to a thin film of yttrium iron garnet, exploiting the non-linear spin-wave dynamics of the magnet.
- Joris J. Carmiggelt
- , Iacopo Bertelli
- & Toeno van der Sar
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Article
| Open AccessConstraints on exotic spin-velocity-dependent interactions
Exotic spin-dependent force are among the possible extensions of the Standard Model that can be probed by precision measurements. Here, the authors use a spin-exchange-relaxation free (SERF) K-Rb-21Ne comagnetometer to improve limits on spin- and velocity dependent forces.
- Kai Wei
- , Wei Ji
- & Dmitry Budker
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Article
| Open AccessImproved bounds on Lorentz violation from composite pulse Ramsey spectroscopy in a trapped ion
Breaking of Lorentz symmetry is related to the unification of fundamental forces and the extension of the standard model. Here the authors provide updated bounds on the Lorentz violation, by using measurements with trapped Yb+ ion, that represent an improvement over existing results.
- Laura S. Dreissen
- , Chih-Han Yeh
- & Tanja E. Mehlstäubler
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Article
| Open AccessQuantum metrology with imperfect measurements
The effects of detection noise on quantum metrology performances have not been rigorously investigated yet. Here, the authors fill this gap by generalising the quantum Fisher information to the case of noisy readout, and showing the consequences the imperfect measurements bring.
- Yink Loong Len
- , Tuvia Gefen
- & Jan Kołodyński
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Article
| Open AccessCoherent dynamics of multi-spin V\({}_{{{{{{{{\rm{B}}}}}}}}}^{-}\) center in hexagonal boron nitride
Understanding the coherent dynamics of electron and nucleus spins in hBN is crucial for their applications as qubits and quantum sensors. Here the authors report room-temperature coherent manipulation of the negatively charged boron vacancy spins in hBN and study their dynamics under weak and strong magnetic fields.
- Wei Liu
- , Viktor Ivády
- & Guang-Can Guo
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Article
| Open AccessQuantum and non-local effects offer over 40 dB noise resilience advantage towards quantum lidar
Sensitivity to noise is currently an obstacle to the use of quantum imaging techniques in real-world scenarios. Here, exploiting non-local cancellation of dispersion on time-frequency entangled photons, the authors show a 43dB improvement in resilience to noise for imaging protocols towards a quantum LiDAR.
- Phillip S. Blakey
- , Han Liu
- & Amr S. Helmy
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Article
| Open AccessHigh field magnetometry with hyperpolarized nuclear spins
Quantum sensors based on NV centers in diamond find applications in high spatial resolution NMR spectroscopy, but their operation is typically limited to low fields. Sahin et al. demonstrate a high-field sensor based on nuclear spins in diamond, where NV centers play a supporting role in optical initialization.
- Ozgur Sahin
- , Erica de Leon Sanchez
- & Ashok Ajoy
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Article
| Open AccessOptical quantum super-resolution imaging and hypothesis testing
Estimating the angular separation between two incoherent sources below the diffraction limit is challenging. Hypothesis testing and quantum state discrimination techniques are used to super-resolve sources of different brightness with a simple optical interferometer.
- Ugo Zanforlin
- , Cosmo Lupo
- & Zixin Huang
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Article
| Open AccessQuantum nonlinear spectroscopy of single nuclear spins
Signals that look the same from their low-order correlations can often be distinguished by looking at higher-order ones. Here, the authors exploit the sensitivity of quantum nonlinear spectroscopy to fourth-order correlations to identify Gaussian noises, random-phased AC fields, and quantum spins.
- Jonas Meinel
- , Vadim Vorobyov
- & J. Wrachtrup
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Article
| Open AccessQuantum-assisted distortion-free audio signal sensing
High sensitivity in quantum sensing comes often at the expense of other figures of merit, usually resulting in distortion. Here, the authors propose a protocol with good sensitivity, readout linearity and high frequency resolution, and benchmark it through signal measurements at audio bands with NV centers.
- Chen Zhang
- , Durga Dasari
- & Jörg Wrachtrup
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Article
| Open AccessDecoherence of V\({}_{{{{{{{{\rm{B}}}}}}}}}^{-}\) spin defects in monoisotopic hexagonal boron nitride
Recently, coherent control of spin defects in hBN has been realized, enabling future applications in quantum sensing technologies. Here the authors perform a systematic study of isotope-dependent spin coherence properties of the negatively-charged boron-vacancy defect in monoisotopic hBN crystals.
- A. Haykal
- , R. Tanos
- & V. Jacques
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Article
| Open AccessScanning gradiometry with a single spin quantum magnetometer
Scanning NV center magnetometry enables imaging of weak magnetic fields at the nanoscale. Huxter et al. achieve an order-of-magnitude improvement in sensitivity by converting a spatial field gradient into an AC field by mechanical oscillations of the sensor, and image stray fields from atomic steps in an antiferromagnet.
- W. S. Huxter
- , M. L. Palm
- & C. L. Degen
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Article
| Open AccessQuantum-enhanced radiometry via approximate quantum error correction
Exotic quantum states can be advantageous for sensing, but are very fragile, so that some form of quantum error correction is needed. Here, the authors show how approximate QEC helps overcoming decoherence due to noise when measuring the excitation population of a receiver mode in a superconducting circuit.
- W. Wang
- , Z.-J. Chen
- & L. Sun
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Article
| Open AccessGround state cooling of an ultracoherent electromechanical system
’Systems with long coherence times are extremely important for the processing of quantum information. To this end the authors present a system able to cool down a resonator to its quantum mechanical ground state harnessing the large coupling between an ultra-coherent mechanical resonator and a superconducting circuit.’
- Yannick Seis
- , Thibault Capelle
- & Albert Schliesser
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Article
| Open AccessParallel detection and spatial mapping of large nuclear spin clusters
Nuclear magnetic resonance imaging at the atomic scale has been limited to detection and localisation of single nuclear spins. Here, the authors extend imaging to large nuclear spin clusters in 3D by combining weak quantum measurements, phase encoding and simulated annealing.
- K. S. Cujia
- , K. Herb
- & C. L. Degen
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Article
| Open AccessSuperresolution concentration measurement realized by sub-shot-noise absorption spectroscopy
Here, the authors use entangled photon pairs as the light source for absorption spectroscopy and demonstrate sub-shot-noise spectra in the entire visible wavelength region. They quantify chemical species in highly diluted solutions with precision beyond the limit of conventional spectroscopy.
- Korenobu Matsuzaki
- & Tahei Tahara
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Article
| Open AccessOptical-domain spectral super-resolution via a quantum-memory-based time-frequency processor
Spectral super-resolution methods generally apply only to laser spectroscopy. Here, thanks to a Gradient Echo Memory with time-frequency processing capabilities, the authors are able to resolve frequency differences with precision below the Fourier limit for narrowband and ultra-low input-light level.
- Mateusz Mazelanik
- , Adam Leszczyński
- & Michał Parniak
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Article
| Open AccessIntrinsic and induced quantum quenches for enhancing qubit-based quantum noise spectroscopy
When trying to characterise a bath coupled to a sensor qubit, one should consider that quantum environments change their properties in response to external perturbations. Here, the authors show how back-action of the qubit on the bath leads to a quench, which can be used to infer the bath spectral function.
- Yu-Xin Wang
- & Aashish A. Clerk
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Article
| Open AccessQuantum enhanced multiple-phase estimation with multi-mode N00N states
N00N states are a key resource in quantum metrology, but the use of their multi-mode extension for multiparameter estimation has been elusive so far. Here, the authors use multi-mode N00N states - with N=2 photons in 4 modes - for multiple-phase estimation saturating the quantum Cramer-Rao bound.
- Seongjin Hong
- , Junaid ur Rehman
- & Hyang-Tag Lim
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Article
| Open AccessSimultaneous bicolor interrogation in thulium optical clock providing very low systematic frequency shifts
There are continuous efforts in improving the stability and systematic shifts of optical clocks. Here the authors demonstrate thulium optical clock utilizing bicolor scheme involving interrogation of both hyperfine levels and they are able to cancel the quadratic Zeeman shift.
- Artem A. Golovizin
- , Dmitry O. Tregubov
- & Nikolai N. Kolachevsky
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Article
| Open AccessEngineering atomic-scale magnetic fields by dysprosium single atom magnets
Single atom magnets on surfaces offer potentially long lived and stable spin states, particular lanthanides, which can be adsorbed onto Magnesium Oxide. Here, the authors report on Dysprosium adsorbed onto Magnesium Oxide, which exhibits large magnetic anisotropy energy, and a spin life time of several days at low temperatures
- A. Singha
- , P. Willke
- & T. Choi
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Article
| Open AccessHeterodyne sensing of microwaves with a quantum sensor
High-resolution microwave detection with NV centers in diamond is currently applicable to signals with frequencies below 10 MHz, thus limiting their range of applications. Here, the authors demonstrate detection of GHz signals with sub-Hz spectral resolution, not limited by the quantum sensor lifetime.
- Jonas Meinel
- , Vadim Vorobyov
- & Jörg Wrachtrup
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Article
| Open AccessTwin-lattice atom interferometry
Atom interferometers can be useful for precision measurement of fundamental constants and sensors of different type. Here the authors demonstrate a compact twin-lattice atom interferometry exploiting Bose-Einstein condensates (BECs) of 87 Rb atoms.
- Martina Gebbe
- , Jan-Niclas Siemß
- & Ernst M. Rasel
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Article
| Open AccessNanoscale electric-field imaging based on a quantum sensor and its charge-state control under ambient condition
Previous work has demonstrated electric-field detection with nitrogen-vacancy centers in diamond; however, nanoscale electric-field imaging has not been shown. Here, the authors use individual nitrogen-vacancy centers to map out electric field contours from a tip of an atomic force microscope with 10 nm resolution.
- Ke Bian
- , Wentian Zheng
- & Ying Jiang
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Article
| Open AccessMetrological complementarity reveals the Einstein-Podolsky-Rosen paradox
Steering reflects the ability to predict measurement results on one side of a quantum-correlated system based on measurements on the other side, which can be phrased as a metrology problem. Here, the authors explore this connection, deriving a general steering criterion based on quantum Fisher information.
- Benjamin Yadin
- , Matteo Fadel
- & Manuel Gessner
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Article
| Open AccessJordan products of quantum channels and their compatibility
Establishing whether two quantum channels are compatible is a fundamental problem in quantum information. Here, the authors prove its equivalence to the quantum state marginal problem, introduce an efficient way to solve both, and draw further connection to the measurement compatibility problem.
- Mark Girard
- , Martin Plávala
- & Jamie Sikora
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Article
| Open AccessUltracold atom interferometry in space
Conducting atom-optical experiments in space is interesting for fundamental physics and challenging due to different environment compared to ground. Here the authors report matter-wave interferometry in space using atomic BECs in a sounding rocket.
- Maike D. Lachmann
- , Holger Ahlers
- & Ernst M. Rasel
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Article
| Open AccessMulti-level quantum noise spectroscopy
Engineering qubits with long coherence times requires the ability to distinguish multiple noise sources, which is not possible with typical two-level qubit sensors. Here the authors utilize the multiple level transitions of a superconducting qubit to characterize two common types of external noise.
- Youngkyu Sung
- , Antti Vepsäläinen
- & William D. Oliver
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Article
| Open AccessA random-walk benchmark for single-electron circuits
Fidelity control is important to quantum metrology and fault-tolerant quantum computation. Here, authors realize clock-controlled transfer of electrons through quantum dots and describe the statistics of accumulated charge by a random-walk model, achieving a benchmark for single-electron circuits.
- David Reifert
- , Martins Kokainis
- & Niels Ubbelohde
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Article
| Open AccessReadout and control of an endofullerene electronic spin
Encasing a single atom within a fullerene (C60) cage can create a robustly packaged single atomic spin system. Here, the authors perform electron paramagnetic resonance on a single encased spin using a diamond NV-center, demonstrating the first steps in controlling single spins in fullerene cages.
- Dinesh Pinto
- , Domenico Paone
- & Klaus Kern
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Article
| Open AccessProspects and challenges for squeezing-enhanced optical atomic clocks
Optical atomic clocks are useful tools for frequency metrology. Here the authors explore the stability of the atomic clocks and the role of the spin squeezed states for the noise reduction in these clocks.
- Marius Schulte
- , Christian Lisdat
- & Klemens Hammerer