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High-mobility and low-power thin-film transistors based on multilayer MoS2 crystals
Molybdenum disulphide offers some tantalizing advantages over graphene as a material with which to fabricate field-effect transistors. Kimet al. present a comprehensive study of field-effect transistors made from multilayer samples of MoS2and find that they can achieve high carrier mobilities.
- Sunkook Kim
- , Aniruddha Konar
- & Kinam Kim
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In situ measurement of exciton energy in hybrid singlet-fission solar cells
Singlet fission converts single singlet excitons into pairs of triplet excitons, and it has been proposed to give additional photocurrent to solar cells. Ehrleret al. use lead selenide nanocrystals of varying sizes to measure the triplet energy in pentacene photovoltaic cells, and achieve efficiencies approaching 5%.
- Bruno Ehrler
- , Brian J. Walker
- & Neil C. Greenham
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| Open AccessAmbient fabrication of flexible and large-area organic light-emitting devices using slot-die coating
Light-emitting electrochromic cells are a promising alternative to organic light-emitting diodes, as their performance is less sensitive to fabrication conditions. Here, a roll-to-roll compatible fabrication of such devices is presented, demonstrating large-area continuous production in ambient conditions.
- Andreas Sandström
- , Henrik F. Dam
- & Ludvig Edman
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Laser-induced ultrafast demagnetization in the presence of a nanoscale magnetic domain network
Understanding ultrafast demagnetisation is key to manipulating magnetic structures on fast timescales, yet laser sources limit the attainable spatial resolution. Here, a soft X-ray high harmonic source enables a high temporal and spatial resolution study of domain demagnetisation in [Co/Pt]30multilayer films.
- Boris Vodungbo
- , Julien Gautier
- & Jan Lüning
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| Open AccessObservation of resistively detected hole spin resonance and zero-field pseudo-spin splitting in epitaxial graphene
Along with its electronic characteristics, the spin properties of graphene have recently received increasing attention in the context of spintronic applications. Using microwave radiation, Maniet al. identify resistively detected spin resonance in monolayer and trilayer graphene sheets and extract the value for the Landé g-factor.
- Ramesh G. Mani
- , John Hankinson
- & Walter A. de Heer
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Skyrmion flow near room temperature in an ultralow current density
Current-induced motion of magnetic nanostructures, such as skyrmions or domain walls, is envisioned as a promising scalable technology for information storage. Yuet al.demonstrate near-room-temperature motion of skyrmions with current densities orders of magnitude lower than previously reported in domain walls.
- X.Z. Yu
- , N. Kanazawa
- & Y. Tokura
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| Open AccessHiggs transition from a magnetic Coulomb liquid to a ferromagnet in Yb2Ti2O7
Quantum spin ice is a magnetic state of matter which can play host to monopole excitations. Using polarized neutron scattering, Changet al. show that the quantum spin ice material ytterbium titanate undergoes a Higgs transition of emergent magnetic monopoles from a Coulomb liquid to a ferromagnetic phase.
- Lieh-Jeng Chang
- , Shigeki Onoda
- & Martin Richard Lees
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| Open AccessLight-induced spiral mass transport in azo-polymer films under vortex-beam illumination
Non-uniform light beams can create patterns in azo-polymer films by inducing mass transport, yet the process is not well understood. Using optical vortex beams, Ambrosioet al. observe the formation of spiral patterns that are surprisingly sensitive to the optical phase, which they explain with a new model.
- Antonio Ambrosio
- , Lorenzo Marrucci
- & Pasqualino Maddalena
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Solderable and electroplatable flexible electronic circuit on a porous stretchable elastomer
The integration of flexible electronics with conventional devices has been hampered by the lack of suitable soldering techniques able to withstand stretching. Jeonget al. use a porous substrate to fabricate biocompatible, stretchable electronics that can be interfaced with commercial components.
- Gi Seok Jeong
- , Dong-Hyun Baek
- & Sang-Hoon Lee
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Topological crystalline insulators in the SnTe material class
Topologically protected states of matter are receiving widespread attention owing to their unusual electronic properties. Using numerical simulations, this study predicts that tin telluride is a physical realization of a new class of materials termed topological crystalline insulators.
- Timothy H. Hsieh
- , Hsin Lin
- & Liang Fu
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Biomimetic layer-by-layer assembly of artificial nacre
Nacre is an organic–inorganic composite biomaterial, which consists of an ordered multilayer structure of crystalline calcium carbonate platelets separated by porous organic layers. Finnemoreet al. present a route to artificial nacre which mimics the natural layer-by-layer biosynthesis.
- Alexander Finnemore
- , Pedro Cunha
- & Ullrich Steiner
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| Open AccessPatterning symmetry in the rational design of colloidal crystals
Patchy colloids are colloidal particles with chemically or physically patterned surfaces that result in complex interactions arising between them. By means of numerical simulations, Romano and Sciortino show that suitably tailored patches can induce the crystallization of patchy colloids into specific crystal structures.
- Flavio Romano
- & Francesco Sciortino
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| Open AccessRoles of icosahedral and crystal-like order in the hard spheres glass transition
The dynamics and structure of the glass transition in liquids is still debated. Using particle-level confocal microscopy, Leocmach and Tanaka investigate supercooled colloidal liquids and distinguish different scenarios for glassy slow dynamics, suggesting that local ordering may only play a minor role.
- Mathieu Leocmach
- & Hajime Tanaka
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| Open AccessStructural correlations in the generation of polaron pairs in low-bandgap polymers for photovoltaics
The electronic and optical properties of polymer semiconductors are largely dictated by their chemical structure. This study examines the nature of the photoexcited states generated in donor–acceptor polymers, and uncovers the dynamics of polaron pairs generation and recombination.
- Raphael Tautz
- , Enrico Da Como
- & Ullrich Scherf
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Realizing a robust practical Majorana chain in a quantum-dot-superconductor linear array
Majorana fermions—the particles renowned for being their own antiparticles—have been proposed as candidates for storing qubits for quantum computers. Sau and Das Sarma propose a method for creating stable Majorana fermions in an array of quantum dots.
- Jay D. Sau
- & S. Das Sarma
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Evidence for charge–vortex duality at the LaAlO3/SrTiO3 interface
Vortex–charge duality is a model that has been proposed for describing the superconducting to insulator transition in disordered thin films. Mehtaet al. report experimental evidence for this duality in the two-dimensional electron gas that arises in LaAlO3/SrTiO3heterostructures.
- M.M. Mehta
- , D.A. Dikin
- & V. Chandrasekhar
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Dynamics of multiple phases in a colossal-magnetoresistive manganite as revealed by dielectric spectroscopy
Correlated electron oxide materials have rich phase diagrams with magnetic or electronic properties. Using a p-n junction configuration, Shenget al. explore the dielectric response of different phases in manganite thin films and uncover their dynamic transport properties.
- Zhigao Sheng
- , Masao Nakamura
- & Yoshinori Tokura
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| Open AccessTwo-dome structure in electron-doped iron arsenide superconductors
The iron pnictides are a class of superconductors that have received widespread interest in recent years. By doping the prototypical material LaFeAsO with hydrogen, this study reveals the existence of a second superconducting dome at higher doping ranges, which arises due to orbital fluctuations.
- Soshi Iimura
- , Satoru Matsuishi
- & Hideo Hosono
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Photoinduced handedness switching in terahertz chiral metamolecules
Chiral metamaterials present interesting ways to manipulate and distinguish between different circular polarizations of light. Zhanget al. realize chiral metamaterials that exhibit photoinduced switching between left- and right-handed circular polarization interactions at terahertz frequencies.
- Shuang Zhang
- , Jiangfeng Zhou
- & Xiang Zhang
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Electronic origin of high-temperature superconductivity in single-layer FeSe superconductor
The exact mechanism for superconductivity in iron-based superconductors remains elusive, but is thought to involve complex interactions between many orbitals. Using angle-resolved photoelectron spectroscopy, Liuet al. report the electronic structure of the single-layer parent compound FeSe.
- Defa Liu
- , Wenhao Zhang
- & X.J. Zhou
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Gate-defined quantum confinement in suspended bilayer graphene
The ability to manipulate single charges is a key requisite for novel nanoelectronic devices. Allenet al. show how to electrostatically confine electrons in suspended bilayer graphene quantum dots by local control of the graphene band structure.
- M. T. Allen
- , J. Martin
- & A. Yacoby
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Tunable conductivity threshold at polar oxide interfaces
The SrTiO3/LaAlO3 system is widely studied because it forms a two-dimensional electron gas at the interface. This study investigates the effects of diluting the LaAlO3 layer with SrTiO3, and finds that the threshold thickness required for the onset of conductivity scales inversely with the fraction of LaAlO3, suggesting an intrinsic origin for the electron gas.
- M.L. Reinle-Schmitt
- , C. Cancellieri
- & P.R. Willmott
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| Open AccessRobust spin crossover and memristance across a single molecule
Switches made up of single molecules form the basis for the concept of molecular electronics. Miyamachiet al.demonstrate that an iron-based spin crossover molecule can be switched between different spin states, provided it is decoupled from a metallic substrate by a thin insulating layer.
- Toshio Miyamachi
- , Manuel Gruber
- & Wulf Wulfhekel
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Critical thickness for ferromagnetism in LaAlO3/SrTiO3 heterostructures
The interface within heterostructures consisting of LaAlO3 and SrTiO3 has been reported to give rise to magnetism, in addition to a two-dimensional electron gas. Kalisky et al. observe that magnetism can occur only above a critical thickness, and that it occurs in heterogeneous patches.
- Beena Kalisky
- , Julie A. Bert
- & Kathryn A. Moler
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Spatial complexity due to bulk electronic nematicity in a superconducting underdoped cuprate
Recent investigations of high-temperature superconductors suggest rotational symmetry is broken in the pseudogap and superconducting states. This theoretical study examines experimental data obtained for a cuprate system known as Dy-Bi2212, and concludes the nematic state extends into the bulk.
- B. Phillabaum
- , E.W. Carlson
- & K.A. Dahmen
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An ultrafast nickel–iron battery from strongly coupled inorganic nanoparticle/nanocarbon hybrid materials
Fast rechargeable batteries made from low-cost and abundant electrode materials are attractive for energy storage. Wanget al. develop an ultrafast Ni–Fe battery with carbon/inorganic hybrid electrodes in which the charge and discharge rates are nearly 1,000-fold higher than traditional Ni–Fe batteries.
- Hailiang Wang
- , Yongye Liang
- & Hongjie Dai
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Three-dimensional nanonetworks for giant stretchability in dielectrics and conductors
Stretchable electronics based on conducting polymers offer new opportunities for designing flexible technologies. Parket al. build three-dimensional nanostructures from elastomers soaked with liquid metal to produce stretchable conductors with greatly improved strain properties over solid films.
- Junyong Park
- , Shuodao Wang
- & Seokwoo Jeon
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Dynamic Jahn–Teller effect in the parent insulating state of the molecular superconductor Cs3C60
Expanded alkali fullerides are molecular superconductors with a Mott parent insulating state. Kluppet al.use infrared spectroscopy to detect the molecular Jahn–Teller distortion of fulleride ions and establish its relevance to strongly correlated superconductivity.
- Gyöngyi Klupp
- , Péter Matus
- & Kosmas Prassides
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| Open AccessLifetime blinking in nonblinking nanocrystal quantum dots
Nanocrystal quantum dots can exhibit photoluminescence blinking, where the intensity of the emitted light fluctuates due to random charging and discharging. Gallandet al.study thick shell nanocrystals and find that the photoluminescence lifetime can also undergo blinking, without intensity changes.
- Christophe Galland
- , Yagnaseni Ghosh
- & Victor I. Klimov
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| Open AccessRobust absolute magnetometry with organic thin-film devices
Magnetometers based on organic magnetoresistance are limited by narrow sensitivity ranges, degradation and temperature fluctuations. Bakeret al. demonstrate a magnetic resonance-based organic thin film magnetometer, which overcomes these drawbacks by exploiting the metrological nature of magnetic resonance.
- W.J. Baker
- , K. Ambal
- & C. Boehme
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| Open AccessAtomic scale dynamics of ultrasmall germanium clusters
Ultrasmall clusters of atoms form the building blocks of many nanoscale materials. Using a combination of aberration-corrected transmission electron microscopy and numerical simulations, this study uncovers the geometry of these clusters in three dimensions.
- S. Bals
- , S. Van Aert
- & G. Van Tendeloo
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| Open AccessUsing light transmission to watch hydrogen diffuse
Understanding hydrogen diffusion in metals is a challenge because of limited access to spatial evolution of the concentration profiles. Using time- and spatially resolved optical measurements, Palssonet al. determine the diffusion rate of hydrogen by directly monitoring its transit through a vanadium thin film.
- Gunnar K. Pálsson
- , Andreas Bliersbach
- & Björgvin Hjörvarsson
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Anomalous high capacitance in a coaxial single nanowire capacitor
Devices made up of nanowires offer promise for a range of electronic, photonic and energy applications. Liuet al. fabricate a miniature capacitor by employing a thin layer of Cu2O as a separator between layers of carbon and copper.
- Zheng Liu
- , Yongjie Zhan
- & Pulickel M. Ajayan
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| Open AccessValley-selective circular dichroism of monolayer molybdenum disulphide
The monolayer transition-metal dichalcogenide molybdenum disulphide has recently attracted attention owing to its distinctive electronic properties. Cao and co-workers present numerical evidence suggesting that circularly polarized light can preferentially excite a single valley in the band structure of this system.
- Ting Cao
- , Gang Wang
- & Ji Feng
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Orbital switching in a frustrated magnet
Thed orbitals of transition metal compounds influence their crystallographic and physical properties. This study reports a unique structural transition in single crystals of the S=1/2 kagomé antiferromagnet, volborthite, whereby an unpaired electron 'switches' from one dorbital to another upon cooling.
- Hiroyuki Yoshida
- , Jun-ichi Yamaura
- & Zenji Hiroi
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Logic gates based on ion transistors
Transistors based on ions, as opposed to electrons, offer the promise of bridging the gap between technological and biological systems. Tybrandtet al. present logic gates based on ion bipolar junction transistors that operate at concentrations compatible with biological systems.
- Klas Tybrandt
- , Robert Forchheimer
- & Magnus Berggren
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| Open AccessStable magnetostructural coupling with tunable magnetoresponsive effects in hexagonal ferromagnets
The coupling that occurs between the structural and the magnetic properties of magnetic materials leads to a host of magnetoresponsive effects that are useful for potential technological applications. Here, a strong magnetostructural coupling that persists over a wide temperature range is reported in MnNiGe:Fe alloys.
- Enke Liu
- , Wenhong Wang
- & Frank de Boer
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| Open AccessElectric-field control of domain wall motion in perpendicularly magnetized materials
The motion of domain walls in magnetic materials characterized by a perpendicular axis of magnetization is a promising means of controlling information in future memory and logic devices. Schellekenset al. show the velocity of domain walls in such systems can be controlled by using an applied electric field.
- A.J. Schellekens
- , A. van den Brink
- & B. Koopmans
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| Open AccessSuperionic glass-ceramic electrolytes for room-temperature rechargeable sodium batteries
Rechargeable solid-state batteries are promising sources of energy for a range of applications. Hayashiet al. examine the electrochemistry of solid-state sodium batteries, and present an electrolyte that operates at room temperature.
- Akitoshi Hayashi
- , Kousuke Noi
- & Masahiro Tatsumisago
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Spin-motive force due to a gyrating magnetic vortex
The electromotive force is a well established phenomenon that is induced by a varying magnetic field. Here, Tanabeet al. report a compelling experimental confirmation of its spin-induced analogue, the spinmotive force.
- K. Tanabe
- , D. Chiba
- & T. Ono
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Closed network growth of fullerenes
The formation mechanisms of fullerenes remain unclear. This study shows that fullerenes self-assemble through a closed network growth mechanism in which atomic carbon and C2are incorporated into the growing closed cages.
- Paul W. Dunk
- , Nathan K. Kaiser
- & Harold W. Kroto
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| Open AccessResonant magnetic exciton mode in the heavy-fermion antiferromagnet CeB6
Resonant magnetic excitations are common in unconventional superconductors, but the mechanism for their formation is elusive. Using inelastic neutron scattering, this study finds similar excitations in the non-superconducting heavy-fermion metal CeB6, suggesting common behaviour between the two ground states.
- G. Friemel
- , Yuan Li
- & D.S. Inosov
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Giant nonlinear optical activity in a plasmonic metamaterial
Light propagating in a medium can undergo polarization rotation, an effect that depends on light intensity and chiral properties. Renet al. report polarization rotation in a plasmonic metamaterial with million-fold stronger nonlinearity than that found in natural crystals.
- Mengxin Ren
- , Eric Plum
- & Nikolay I. Zheludev
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| Open AccessSwitching of macroscopic molecular recognition selectivity using a mixed solvent system
Self-assembly via molecular recognition events is used in the production of functionalized materials. This Article reports that the macroscopic assembly of polyacrylamide gels can be controlled by changing the composition of a mixed solvent system.
- Yongtai Zheng
- , Akihito Hashidzume
- & Akira Harada
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Phase fluctuations and the absence of topological defects in a photo-excited charge-ordered nickelate
Time- and momentum-resolved spectroscopy gives dynamical information on complex materials, enabling disentanglement of their coupled degrees of freedom. Using time-resolved X-ray diffraction at a free electron laser, Leeet al. investigate the charge order parameter in a striped nickelate.
- W.S. Lee
- , Y.D. Chuang
- & Z. Hussain
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| Open AccessEnamel-like apatite crown covering amorphous mineral in a crayfish mandible
The compositional makeup of skeletons and teeth in invertebrates and vertebrates is generally different. This study examines the material composition and properties of freshwater crayfish mandibles and finds, in an unusual case of convergent evolution, that they are composed of an apatite layer that is similar to mammalian enamel.
- Shmuel Bentov
- , Paul Zaslansky
- & Barbara Aichmayer
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| Open AccessNanotomy-based production of transferable and dispersible graphene nanostructures of controlled shape and size
Current top-down and bottom-up syntheses of graphene nanostructures suffer from low yields or do not produce structures with different and controlled shapes. Here, monodisperse graphene shapes are produced by diamond-edge cutting of pyrolytic graphite followed by exfoliation.
- Nihar Mohanty
- , David Moore
- & Vikas Berry
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Transforming moiré blisters into geometric graphene nano-bubbles
Strain engineering has been proposed as a promising strategy for manipulating the electronic properties of graphene. This scanning tunnelling microscopy study demonstrates the feasibility of controlling strain patterns in graphene down to the nanoscale.
- Jiong Lu
- , A.H. Castro Neto
- & Kian Ping Loh
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| Open AccessGraphene quilts for thermal management of high-power GaN transistors
Electronic and optoelectronic devices based on gallium nitride suffer from self-heating arising as a result of their operation. This study presents and demonstrates a strategy for managing this problem that relies on graphene quilts which dissipate the heat away.
- Zhong Yan
- , Guanxiong Liu
- & Alexander A. Balandin