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| Open AccessA large-strain and ultrahigh energy density dielectric elastomer for fast moving soft robot
Dielectric elastomer actuators require high driving electric fields to achieve high performances for soft robots due to their low dielectric constant and high stiffness. Here, the authors introduce polar fluorinated groups and nanodomains aggregated by long alkyl side chains into the dielectric elastomer design to overcome these issues and develop fast soft robots.
- Wenwen Feng
- , Lin Sun
- & Chao Wang
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| Open AccessAdvancing interactive systems with liquid crystal network-based adaptive electronics
There is significant interest in developing electronic units that can perform sensing, signal processing, and actuation functions independently, similar to biological systems. Lyu et al. develop electronic units based on liquid crystal oligomer networks that exhibit adaptive behavior in response to environmental stimuli such as light and heat.
- Pengrong Lyu
- , Dirk J. Broer
- & Danqing Liu
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| Open AccessMagnetic steering continuum robot for transluminal procedures with programmable shape and functionalities
Interaction with surrounding lumina leads to potential medical risks in transluminal procedures. Here, the authors report a magnetic steering continuum robot that achieve autonomous shaping without the need for environmental interaction.
- Liyang Mao
- , Peng Yang
- & Hui Xie
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| Open AccessHighly efficient in crystallo energy transduction of light to work
Crystals are known to have a range of responses to light, but multiple responses in the same material are rare. Here, the authors report different mechanical effects in response to light across three polymorphs as a result of a dimerization reaction.
- Jiawei Lin
- , Jianmin Zhou
- & Junbo Gong
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Article
| Open AccessMultiple hydrogen-bonding induced nonconventional red fluorescence emission in hydrogels
The development of fluorescent polymer hydrogels without the use of extended pi-conjugation is challenging. Here, the authors report the use of clustering-trigger emission to give red fluorescence on boiling polymer hydrogels, with tuneable emission properties.
- Jiayu Wu
- , Yuhuan Wang
- & Feng Zhou
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| Open AccessEstablishing superfine nanofibrils for robust polyelectrolyte artificial spider silk and powerful artificial muscles
Spider silk has desirable properties, but these are hard to replicate with artificial materials. Here, the authors report a polyelectrolyte artificial spider silk, with control over dissociation of the polymer chains by introduction of ions, and thermally driven supercontraction.
- Wenqian He
- , Meilin Wang
- & Zunfeng Liu
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Article
| Open AccessHeight-renderable morphable tactile display enabled by programmable modulation of local stiffness in photothermally active polymer
The controllability of deformation height in reconfigurable touch displays currently limits their deliverable information. Hwang et al. present a light-triggered morphable tactile display enabling generation of refreshable, height-adjustable, and latchable 3D topologies with varying textures on a thin film surface.
- Inwook Hwang
- , Seongcheol Mun
- & Sungryul Yun
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| Open AccessContribution of irreversible non-180° domain to performance for multiphase coexisted potassium sodium niobate ceramics
Seeking eco-friendly materials with equivalent performance to lead-based piezoelectric materials remains an urgent demand. Here, the authors design potassium–sodium niobate-based lead-free piezoelectric materials with large potential.
- Bo Wu
- , Lin Zhao
- & Ke Wang
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Article
| Open AccessSpeaking without vocal folds using a machine-learning-assisted wearable sensing-actuation system
Addressing challenges in voice disorders, the authors present a self-powered, wearable sensor-actuator system based on magnetoelasticity. This innovation enables assisted speaking by capturing laryngeal movements and translating them into voice signals, bypassing the vocal folds.
- Ziyuan Che
- , Xiao Wan
- & Jun Chen
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Article
| Open AccessCrystallization of piezoceramic films on glass via flash lamp annealing
Direct growth of piezoelectric oxides on glass is difficult due to high processing temperatures. Here, the authors demonstrate a flash lamp process for the growth of films on various glasses in a few seconds only. The films have piezoelectric e33,f of −5 C m−2 and can be used in haptic devices.
- Longfei Song
- , Juliette Cardoletti
- & Sebastjan Glinšek
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Article
| Open AccessSelf-regulated reversal deformation and locomotion of structurally homogenous hydrogels subjected to constant light illumination
Environmentally adaptive hydrogels have great potential as soft robotics but achieving self-regulated reversal shape deformation in homogenous hydrogels under a constant stimulus is challenging. Here, the authors report responsive hydrogels functionalized with two photoswitchable spiropyrans that exhibit self-regulated transient deformation reversal when subjected to constant illumination.
- Kexin Guo
- , Xuehan Yang
- & Chuang Li
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Article
| Open AccessStenus-inspired, swift, and agile untethered insect-scale soft propulsors
Inspired by the swift swingable abdomen, conducting canals, and body setae of Stenus comma, the authors present a swift, agile untethered insect-scale soft propulsor, offering new insights into systematically bio-inspired artificial soft robots.
- Xingxing Ke
- , Haochen Yong
- & Zhigang Wu
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| Open AccessDesigning transparent piezoelectric metasurfaces for adaptive optics
Most multi-degrees-of-freedom systems are composed of several piezoelectric stacks, leading to cumbersome and complicated structures. Here, the authors propose a piezo metasurface to achieve various types of high strains in a wide frequency range.
- Liao Qiao
- , Xiangyu Gao
- & Fei Li
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Article
| Open AccessFunctionally antagonistic polyelectrolyte for electro-ionic soft actuator
Electro-active ionic soft actuators generally present slow responses and poor durability when are applied as artificial muscles. Here, the authors describe a polyelectrolyte membrane based on the assembly of Nafion molecules into micelles with efficient ionic conducting pathways for electro-ionic soft actuators and soft robotics with fast responses and long durability.
- Van Hiep Nguyen
- , Saewoong Oh
- & Il-Kwon Oh
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| Open AccessTunable and parabolic piezoelectricity in hafnia under epitaxial strain
The sign of longitudinal piezoelectric coefficients is typically positive. Here, the authors tune the sign of the linear piezoelectric coefficient of HfO2 from positive to negative via epitaxial strain, finding nonlinear and parabolic piezoelectric behaviors at tensile epitaxial strain.
- Hao Cheng
- , Peijie Jiao
- & Yurong Yang
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Article
| Open AccessOctopus-inspired deception and signaling systems from an exceptionally-stable acene variant
The design of multifunctional platforms with tunable spectroscopic and fluorescent properties that span the ultraviolet, visible, and near-infrared spectral regions remains challenging. Here, the authors report an actuator-type system that leverages a readily-prepared, easily-processable, and exceptionally-stable nonacene-like molecule to achieve multiple complementary dynamic operating modes.
- Preeta Pratakshya
- , Chengyi Xu
- & Alon A. Gorodetsky
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Article
| Open AccessPhysics-aware differentiable design of magnetically actuated kirigami for shape morphing
A differentiable design framework that integrates both geometrical and magnetomechanical analyses to inversely program the shape morphing in magnetically actuated kirigami is proposed, achieving intricate shapes and multistate transitions.
- Liwei Wang
- , Yilong Chang
- & Wei Chen
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Article
| Open AccessUltraflexible, cost-effective and scalable polymer-based phase change composites via chemical cross-linking for wearable thermal management
Jing et al. report a cost-effective chemical cross-linking method for synthesizing ultraflexible polymer-based phase change composites with 3D crosslinked networks and further demonstrate portable applications for wearable thermal management.
- Yaoge Jing
- , Zhengchuang Zhao
- & Tingxian Li
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Article
| Open Access3D-printed liquid metal polymer composites as NIR-responsive 4D printing soft robot
“The combination of stimuli responsive nanomaterials and 3D printing leads interesting applications in the fields of soft robots and actuators. Here, the authors present a 3D printing approach for the fabrication of liquid metal nanoparticles-polymer composites acting as light controlled soft robots which can lift weights, grasp and release items”.
- Liwen Zhang
- , Xumin Huang
- & Ruirui Qiao
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| Open AccessAutonomous nanorobots with powerful thrust under dry solid-contact conditions by photothermal shock
Optically trapping objects, marked by Nobel Prizes in 1997 and 2018 for applications in vacuum and liquids, remains challenging on solid surfaces. Here, the authors demonstrate a breakthrough by using photothermal-shock tweezers and explore nano-conventional robot applications
- Zhaoqi Gu
- , Runlin Zhu
- & Fuxing Gu
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| Open AccessHigh speed underwater hydrogel robots with programmable motions powered by light
Underwater soft robots made of stimuli-responsive shape-changing hydrogels generally present low actuation speed which is limited by the water diffusion between hydrogels and their surrounding environment. Here, the authors develop dynamic hydrogel robots with a fast and switchable actuation based on a thermally driven chain conformation change after mechanical programming.
- Chujun Ni
- , Di Chen
- & Qian Zhao
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Article
| Open AccessLead-free Zr-doped ceria ceramics with low permittivity displaying giant electrostriction
Electrostrictors are materials that develop mechanical strain proportional to the square of the applied electric field. Here authors report. Zr-doped-Ceria as a new lead-free electrostrictive material with a similar electrostriction coefficient to the best electrostrictor material currently in use.
- Maxim Varenik
- , Boyuan Xu
- & Igor Lubomirsky
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| Open AccessReconfigurable self-assembly of photocatalytic magnetic microrobots for water purification
Microrobot collectives promise new functions beyond individuals’ capability. Here, nature-inspired reconfigurable self-assembly of microrobots was created, driven by their photocatalytic and magnetic properties, showing potential application in water purification.
- Mario Urso
- , Martina Ussia
- & Martin Pumera
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Article
| Open AccessProgramming actuation onset of a liquid crystalline elastomer via isomerization of network topology
Tuning actuation temperatures of liquid crystalline elastomers can help control actuation behaviour, but normally cannot be altered following the synthesis of the material. Here, the authors report the development of an elastomer with varying actuation temperature depending on the conditions.
- Guancong Chen
- , Haijun Feng
- & Qian Zhao
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| Open Access4D Optical fibers based on shape-memory polymers
The authors demonstrate here a method for the production of arbitrarily long, light-guiding microstructured fibers with shape-memory properties. The showcased design of adaptative fibers here holds potential for the development of functional actuators and sensors.
- Clément Strutynski
- , Marianne Evrard
- & Frédéric Smektala
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| Open AccessSelf-protection soft fluidic robots with rapid large-area self-healing capabilities
The soft fluidic robots designed so far are lacking intelligent self-protection and present poor fluidic power source. Here, the authors report soft fluidic robots that integrate soft electrohydrodynamic pumps, healing electrofluids, actuators and E-skins endowing them with self-sensing, self-judgment, and self-heating behaviours for rapid self-healing.
- Wei Tang
- , Yiding Zhong
- & Jun Zou
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| Open AccessBi-enzymatic chemo-mechanical feedback loop for continuous self-sustained actuation of conducting polymers
Owing to their interesting applications from soft robotics to biomedicine, methodologies to produce artificial actuators are desirable. Herein the authors develop an autonomous soft bioelectrochemical actuator with self-sustained motion triggered by spontaneous enzymatic reactions.
- Serena Arnaboldi
- , Gerardo Salinas
- & Alexander Kuhn
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| Open AccessProgrammable nanocomposites of cellulose nanocrystals and zwitterionic hydrogels for soft robotics
Soft robots made of hydrogels with anisotropic and shape-change properties offer interesting design opportunities. Here, the authors report zwitterionic hydrogels and anisotropic cellulose nanocrystals composites in which the shear-induced alignment of cellulose nanocrystals allows for the development of shape-change programmable miniature robots.
- Rasool Nasseri
- , Negin Bouzari
- & Hamed Shahsavan
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Article
| Open AccessEmbedded shape morphing for morphologically adaptive robots
Sun et al. introduce a novel embedded shape-morphing method, enabling robots to adapt to environments or tasks by changing their morphologies through embedded actuation, sensing, and shape locking, all within a robot’s body.
- Jiefeng Sun
- , Elisha Lerner
- & Jianguo Zhao
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Article
| Open AccessBioinspired rotary flight of light-driven composite films
Light-driven actuators have great potential in different types of applications but is still challenging to apply them in flying devices owing to their slow response, small deflection and force output. Here, the authors report a rotary flying photoactuator with fast rotation and rapid response.
- Dan Wang
- , Zhaomin Chen
- & Metin Sitti
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| Open AccessCoaxially printed magnetic mechanical electrical hybrid structures with actuation and sensing functionalities
Achieving hybrid magnetic actuation, energy transfer and somatosensory actuation functions in soft electromagnetic devices is a challenge. Here, Zhang et. al. present a hybrid core-sheath fiber and use a one-step coaxial printing method to create complex 2D/3D structures with multimodal functionalities.
- Yuanxi Zhang
- , Chengfeng Pan
- & Lelun Jiang
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| Open AccessPlug & play origami modules with all-purpose deformation modes
Actuators provide robot locomotion and manipulation, but most are limited by their number of motion types and coupled motions. Here, Zhang et. al. present an origami actuation module based on a modified Kresling pattern with pneumatically-driven pouches, thus enabling seven motion modes in one module.
- Chao Zhang
- , Zhuang Zhang
- & Hanqing Jiang
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Article
| Open AccessThermally trainable dual network hydrogels
Trainable responsive materials have received research interests for future adaptive and intelligent material systems but to date trainable responsive materials only allow one direction of functionality change. Here, the authors demonstrate thermally trainable hydrogel systems consisting of two thermoresponsive polymers, where the volumetric response of the system upon phase transitions enhances or decreases through a training process above a certain threshold temperature.
- Shanming Hu
- , Yuhuang Fang
- & Hang Zhang
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Article
| Open AccessPen-drawn Marangoni swimmer
Marangoni swimmers have high relative speed, considering the body length and absence of a mechanical system but the fabricating is complex. Song et al. transform simple pen strokes into dynamic, programmable robots that can ‘swim’ with striking versatility.
- Seo Woo Song
- , Sumin Lee
- & Jiyun Kim
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| Open AccessEnabling liquid crystal elastomers with tunable actuation temperature
Isotropization temperature determines the temperature at which Liquid Crystals Elastomer (LCE) material actuates. Here, the authors give a general strategy based on dynamic covalent bonds for tuning the isotropization temperature for LCEs.
- Yanjin Yao
- , Enjian He
- & Yan Ji
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| Open AccessLight-driven dandelion-inspired microfliers
Insect-scale untethered micro aerial vehicles such as artificial dandelion devices suffer from high flight randomness and inadequate controllability. Chen et al. design and fabricate an untethered dandelion-inspired microflier, which is spatially and temporally controlled by an ultralight and supersensitive light-driven bimorph soft actuator.
- Yuanhao Chen
- , Cristian Valenzuela
- & Wei Feng
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| Open AccessBioinspired soft robots based on organic polymer-crystal hybrid materials with response to temperature and humidity
Response by mechanical deformation to give actuation is essential in the design of soft robots. Here, the authors demonstrate that combining organic molecular crystals with polymers makes it possible to create materials with susceptible properties to changes in temperature and humidity.
- Xuesong Yang
- , Linfeng Lan
- & Hongyu Zhang
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Article
| Open AccessA supramolecular gel-elastomer system for soft iontronic adhesives
Electroadhesion in soft robotics provides controllable interfacial attraction for robotic functionalities but materials selection is limited. Here, Gao et. al. present an iontronic adhesive to design a soft iontronic gripper with self-healability, tunable adhesion at reduced voltages and rapid release.
- Dace Gao
- , Gurunathan Thangavel
- & Pooi See Lee
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Article
| Open AccessLight-driven peristaltic pumping by an actuating splay-bend strip
Small-scale manipulation of liquids is being controlled with bulky pumps or power sources. Dradrach et al. show a light-driven pumping of micro-liter liquid using a centimeter-long liquid crystal elastomer strip.
- Klaudia Dradrach
- , Michał Zmyślony
- & Piotr Wasylczyk
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| Open AccessOrigami-based integration of robots that sense, decide, and respond
Origami-inspired engineering has enabled intelligent materials and structures to react to environments, yet a complete sense-decide-act autonomous loop is still challenging. Yan et al. introduce autonomous origami robots by embedding sensing, computing, and actuating in compliant, conductive materials.
- Wenzhong Yan
- , Shuguang Li
- & Ankur Mehta
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Article
| Open AccessPolyvinyl chloride-based dielectric elastomer with high permittivity and low viscoelasticity for actuation and sensing
Dielectric elastomers (DEs) are widely used in soft actuators but existing DE actuators often require high driving electrical fields. Here the authors demonstrate that introducing cyanoethyl cellulose into plasticized PVC gel confers high dielectric permittivity and allows the fabrication of elastomer actuators with high permittivity and low viscoelasticity
- Jianjian Huang
- , Xiaodie Zhang
- & Dongjie Guo
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Article
| Open AccessPolymer-dispersed liquid crystal elastomers as moldable shape-programmable material
Development of Soft shape-memory materials is often limited to the synthesis of two-dimensional specimens and rely on bending mechanisms and scaffolding topology to perform three-dimensional morphing. Here, the authors demonstrate a shape-memory composite material made from main-chain liquid crystal elastomer microparticles dispersed in a silicone polymer matrix which enables molding into full-volume objects of any shape or size.
- Matej Bobnar
- , Nikita Derets
- & Andraž Rešetič
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Article
| Open AccessBio-inspired magnetic-driven folded diaphragm for biomimetic robot
Soft robotics holds promise for realizing easy control over complex locomotion and deformation. Lin et al. report an earthworm-inspired untethered magnetic robot that consists one-piece-mold folded diaphragm to achieve large three-dimensional deformation with inside-volume change capability.
- Dezhao Lin
- , Fan Yang
- & Ruihong Li
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Article
| Open AccessHigh-performance Marangoni hydrogel rotors with asymmetric porosity and drag reduction profile
Utilizing the Marangoni effect, miniaturized machineries can be endowed with self-propulsion. Here, the authors report high-performance Marangoni hydrogel rotors with asymmetric porosity and drag reduction profile and demonstrate multiple potential functionalities.
- Hao Wu
- , Yiyu Chen
- & Dong Wu
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Article
| Open AccessSelf-rolling of vanadium dioxide nanomembranes for enhanced multi-level solar modulation
In this work, authors demonstrate a smart window combining mechanochromism with thermochromism by self-rolling of VO2 nanomembranes to modulate in-door temperature self-adapted to seasons and climate with high efficiency.
- Xing Li
- , Cuicui Cao
- & Yongfeng Mei
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Article
| Open AccessFinger-palm synergistic soft gripper for dynamic capture via energy harvesting and dissipation
Soft materials are promising candidates for robotics with outstanding performance and functionality. Zhang et al. present an energy harvesting and dissipation mechanism and describe the development of a soft gripper designed for capturing objects with high kinetic energy.
- Yin Zhang
- , Wang Zhang
- & Wei Pu
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| Open AccessDesign of large-span stick-slip freely switchable hydrogels via dynamic multiscale contact synergy
Switching between adhesive and non-adhesive states is important to design materials with on-demand adhesion properties but realizing reversible switching on large scale remains challenging. Here, the authors report the design of a hydrogel demonstrating rapid and reversibly switch between slippery and sticky states.
- Zhizhi Zhang
- , Chenxi Qin
- & Feng Zhou
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Article
| Open AccessPhotothermal modulated dielectric elastomer actuator for resilient soft robots
Tough and healable elastomers are promising materials to realize resilient soft robots but mechanical enhancements often lead to higher stiffness that deteriorates actuation strains. Here, the authors introduce liquid metal nanoparticles into carboxyl polyurethane elastomer to sensitize a dielectric elastomer actuator with responsiveness to electric fields and NIR light.
- Matthew Wei Ming Tan
- , Hyunwoo Bark
- & Pooi See Lee
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Article
| Open AccessMiniaturized electromechanical devices with multi-vibration modes achieved by orderly stacked structure with piezoelectric strain units
Most piezoelectric coefficients in piezoelectric ceramics are zero, resulting in many piezoelectric vibration modes cannot be excited. Here, the authors propose an orderly stacked structure to achieve all nonzero piezoelectric coefficients.
- Jinfeng Liu
- , Xiangyu Gao
- & Fei Li